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Register a new userHigher-order exchange interactions in two-dimensional magnets
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Magnetism in recently discovered van der Waals materials has opened new avenues in the study of fundamental spin interactions in truly two-dimensions. A paramount question is what effect higher-order interactions beyond bilinear Heisenberg exchange have on the magnetic properties of few-atom thick compounds. Here we demonstrate that biquadratic exchange interactions, which is the simplest and most natural form of non-Heisenberg coupling, assume a key role in the magnetic properties of layered magnets. Using a combination of nonperturbative analytical techniques, non-collinear first-principles methods and classical Monte Carlo calculations that incorporate higher-order exchange, we show that several quantities including magnetic anisotropies, spin-wave gaps and topological spin-excitations are intrinsically renormalized leading to further thermal stability of the layers. We develop a spin Hamiltonian that also contains antisymmetric exchanges (e.g. Dzyaloshinskii-Moriya interactions) to successfully rationalize numerous observations currently under debate, such as the non-Ising character of several compounds despite a strong magnetic anisotropy, peculiarities of the magnon spectrum of 2D magnets, and the discrepancy between measured and calculated Curie temperatures. Our results lay the foundation of a universal higher-order exchange theory for novel 2D magnetic design strategies.
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Three-dimensional topological (crystalline) insulators are materials with an insulating bulk, but conducting surface states which are topologically protected by time-reversal (or spatial) symmetries. Here, we extend the notion of three-dimensional topological insulators to systems that host no gapless surface states, but exhibit topologically protected gapless hinge states. Their topological character is protected by spatio-temporal symmetries, of which we present two cases: (1) Chiral higher-order topological insulators protected by the combination of time-reversal and a four-fold rotation symmetry. Their hinge states are chiral modes and the bulk topology is $mathbb{Z}_2$-classified. (2) Helical higher-order topological insulators protected by time-reversal and mirror symmetries. Their hinge states come in Kramers pairs and the bulk topology is $mathbb{Z}$-classified. We provide the topological invariants for both cases. Furthermore we show that SnTe as well as surface-modified Bi$_2$TeI, BiSe, and BiTe are helical higher-order topological insulators and propose a realistic experimental setup to detect the hinge states.
We investigate higher-order Weyl semimetals (HOWSMs) having bulk Weyl nodes attached to both surface and hinge Fermi arcs. We identify a new type of Weyl node, that we dub a $2nd$ order Weyl node, that can be identified as a transition in momentum space in which both the Chern number and a higher order topological invariant change. As a proof of concept we use a model of stacked higher order quadrupole insulators to identify three types of WSM phases: $1st$-order, $2nd$-order, and hybrid-order. The model can also realize type-II and hybrid-tilt WSMs with various surface and hinge arcs. Moreover, we show that a measurement of charge density in the presence of magnetic flux can help identify some classes of $2nd$ order WSMs. Remarkably, we find that coupling a $2nd$-order Weyl phase with a conventional $1st$-order one can lead to a hybrid-order topological insulator having coexisting surface cones and flat hinge arcs that are independent and not attached to each other. Finally, we show that periodic driving can be utilized as a way for generating HOWSMs. Our results are relevant to metamaterials as well as various phases of Cd$_3$As$_2$, KMgBi, and rutile-structure PtO$_2$ that have been predicted to realize higher order Dirac semimetals.
In this article we study 3D non-Hermitian higher-order Dirac semimetals (NHHODSMs). Our focus is on $C_4$-symmetric non-Hermitian systems where we investigate inversion ($mathcal{I}$) or time-reversal ($mathcal{T}$) symmetric models of NHHODSMs having real bulk spectra. We show that they exhibit the striking property that the bulk and surfaces are anti-PT and PT symmetric, respectively, and so belong to two different topological classes realizing a novel non-Hermitian topological phase which we call a emph{hybrid-PT topological phases}. Interestingly, while the bulk spectrum is still fully real, we find that exceptional Fermi-rings (EFRs) appear connecting the two Dirac nodes on the surface. This provides a route to probe and utilize both the bulk Dirac physics and exceptional rings/points on equal footing. Moreover, particularly for $mathcal{T}$-NHHODSMs, we also find real hinge-arcs connecting the surface EFRs. We show that this higher-order topology can be characterized using a biorthogonal real-space formula of the quadrupole moment. Furthermore, by applying Hermitian $C_4$-symmetric perturbations, we discover various novel phases, particularly: (i) an intrinsic $mathcal{I}$-NHHODSM having hinge arcs and gapped surfaces, and (ii) a novel $mathcal{T}$-symmetric skin-topological HODSM which possesses both topological and skin hinge modes. The interplay between non-Hermition and higher-order topology in this work paves the way toward uncovering rich phenomena and hybrid functionality that can be readily realized in experiment.
The study of topological band structures have sparked prominent research interest the past decade, culminating in the recent formulation of rather prolific classification schemes that encapsulate a large fraction of phases and features. Within this context we recently reported on a class of unexplored topological structures that thrive on the concept of {it sub-dimensional topology}. Although such phases have trivial indicators and band representations when evaluated over the complete Brillouin zone, they have stable or fragile topologies within sub-dimensional spaces, such as planes or lines. This perspective does not just refine classification pursuits, but can result in observable features in the full dimensional sense. In three spatial dimensions (3D), for example, sub-dimensional topologies can be characterized by non-trivial planes, having general topological invariants, that are compensated by Weyl nodes away from these planes. As a result, such phases have 3D stable characteristics such as Weyl nodes, Fermi arcs and edge states that can be systematically predicted by sub-dimensional analysis. Within this work we further elaborate on these concepts. We present refined representation counting schemes and address distinctive bulk-boundary effects, that include momentum depended (higher order) edge states that have a signature dependence on the perpendicular momentum. As such, we hope that these insights might spur on new activities to further deepen the understanding of these unexplored phases.
Magnetism in single-side hydrogenated (C$_2$H) and fluorinated (C$_2$F) graphene is analyzed in terms of the Heisenberg model with parameters determined from first principles. We predict a frustrated ground state for both systems, which means the instability of collinear spin structures and sheds light on the absence of a conventional magnetic ordering in defective graphene demonstrated in recent experiments. Moreover, our findings suggest a highly correlated magnetic behavior at low temperatures offering the possibility of a spin-liquid state.
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