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Non-Hermitian Higher-Order Dirac Semimetals

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 Publication date 2021
  fields Physics
and research's language is English




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In this article we study 3D non-Hermitian higher-order Dirac semimetals (NHHODSMs). Our focus is on $C_4$-symmetric non-Hermitian systems where we investigate inversion ($mathcal{I}$) or time-reversal ($mathcal{T}$) symmetric models of NHHODSMs having real bulk spectra. We show that they exhibit the striking property that the bulk and surfaces are anti-PT and PT symmetric, respectively, and so belong to two different topological classes realizing a novel non-Hermitian topological phase which we call a emph{hybrid-PT topological phases}. Interestingly, while the bulk spectrum is still fully real, we find that exceptional Fermi-rings (EFRs) appear connecting the two Dirac nodes on the surface. This provides a route to probe and utilize both the bulk Dirac physics and exceptional rings/points on equal footing. Moreover, particularly for $mathcal{T}$-NHHODSMs, we also find real hinge-arcs connecting the surface EFRs. We show that this higher-order topology can be characterized using a biorthogonal real-space formula of the quadrupole moment. Furthermore, by applying Hermitian $C_4$-symmetric perturbations, we discover various novel phases, particularly: (i) an intrinsic $mathcal{I}$-NHHODSM having hinge arcs and gapped surfaces, and (ii) a novel $mathcal{T}$-symmetric skin-topological HODSM which possesses both topological and skin hinge modes. The interplay between non-Hermition and higher-order topology in this work paves the way toward uncovering rich phenomena and hybrid functionality that can be readily realized in experiment.



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We study non-Hermitian higher-order Weyl semimetals (NHHOWSMs) possessing real spectra and having inversion $mathcal{I}$ ($mathcal{I}$-NHHOWSM) or time-reversal symmetry $mathcal{T}$ ($mathcal{T}$-NHHOWSM). When the reality of bulk spectra is lost, the NHHOWSMs exhibit various configurations of surface Fermi Arcs (FAs) and Exceptional Fermi Rings (EFRs), providing a setup to investigate them on an equal footing. The EFRs only appear in the region between 2nd-order WNs. We also discover Weyl nodes originating from non-Hermicity, called non-Hermitian Weyl nodes (NHWNs). Remarkably, we find T-NHHOWSMs which host only 2nd-order NHWNs, having both surface and hinge FAs protected by the quantized biorthogonal Chern number and quadrupole moment, respectively. We call this intrinsically non-Hermitian phase exceptional HOWSM. In contrast to ordinary WNs, the NHWNs can instantly deform to line nodes, forming a monopole comet. The NHWNs also show exceptional tilt-rigidity, which is a strong resistance towards titling due to attachment to exceptional structures. This phenomenon can be a promising experimental knob. Finally, we reveal the exceptional stability of FAs called exceptional helicity. Surface FAs having opposite chirality can live on the same surface without gapping out each other due to the complex nature of the spectrum. Our work motivates an immediate experimental realization of NHHOWSMs.
We investigate higher-order Weyl semimetals (HOWSMs) having bulk Weyl nodes attached to both surface and hinge Fermi arcs. We identify a new type of Weyl node, that we dub a $2nd$ order Weyl node, that can be identified as a transition in momentum space in which both the Chern number and a higher order topological invariant change. As a proof of concept we use a model of stacked higher order quadrupole insulators to identify three types of WSM phases: $1st$-order, $2nd$-order, and hybrid-order. The model can also realize type-II and hybrid-tilt WSMs with various surface and hinge arcs. Moreover, we show that a measurement of charge density in the presence of magnetic flux can help identify some classes of $2nd$ order WSMs. Remarkably, we find that coupling a $2nd$-order Weyl phase with a conventional $1st$-order one can lead to a hybrid-order topological insulator having coexisting surface cones and flat hinge arcs that are independent and not attached to each other. Finally, we show that periodic driving can be utilized as a way for generating HOWSMs. Our results are relevant to metamaterials as well as various phases of Cd$_3$As$_2$, KMgBi, and rutile-structure PtO$_2$ that have been predicted to realize higher order Dirac semimetals.
Dirac and Weyl semimetals both exhibit arc-like surface states. However, whereas the surface Fermi arcs in Weyl semimetals are topological consequences of the Weyl points themselves, the surface Fermi arcs in Dirac semimetals are not directly related to the bulk Dirac points, raising the question of whether there exists a topological bulk-boundary correspondence for Dirac semimetals. In this work, we discover that strong and fragile topological Dirac semimetals exhibit 1D higher-order hinge Fermi arcs (HOFAs) as universal, direct consequences of their bulk 3D Dirac points. To predict HOFAs coexisting with topological surface states in solid-state Dirac semimetals, we introduce and layer a spinful model of an $s-d$-hybridized quadrupole insulator (QI). We develop a rigorous nested Jackiw-Rebbi formulation of QIs and HOFA states. Employing $ab initio$ calculations, we demonstrate HOFAs in both the room- ($alpha$) and intermediate-temperature ($alpha$) phases of Cd$_{3}$As$_2$, KMgBi, and rutile-structure ($beta$-) PtO$_2$.
Three-dimensional topological (crystalline) insulators are materials with an insulating bulk, but conducting surface states which are topologically protected by time-reversal (or spatial) symmetries. Here, we extend the notion of three-dimensional topological insulators to systems that host no gapless surface states, but exhibit topologically protected gapless hinge states. Their topological character is protected by spatio-temporal symmetries, of which we present two cases: (1) Chiral higher-order topological insulators protected by the combination of time-reversal and a four-fold rotation symmetry. Their hinge states are chiral modes and the bulk topology is $mathbb{Z}_2$-classified. (2) Helical higher-order topological insulators protected by time-reversal and mirror symmetries. Their hinge states come in Kramers pairs and the bulk topology is $mathbb{Z}$-classified. We provide the topological invariants for both cases. Furthermore we show that SnTe as well as surface-modified Bi$_2$TeI, BiSe, and BiTe are helical higher-order topological insulators and propose a realistic experimental setup to detect the hinge states.
Within a Kubo formalism, we study dc transport and ac optical properties of 3D Dirac and Weyl semimetals. Emphasis is placed on the approach to charge neutrality and on the differences between Dirac and Weyl materials. At charge neutrality, the zero-temperature limit of the dc conductivity is not universal and also depends on the residual scattering model employed. However, the Lorenz number L retains its usual value L_0. With increasing temperature, the Wiedemann-Franz law is violated. At high temperatures, L exhibits a new plateau at a value dependent on the details of the scattering rate. Such details can also appear in the optical conductivity, both in the Drude response and interband background. In the clean limit, the interband background is linear in photon energy and always extrapolates to the origin. This background can be shifted to the right through the introduction of a massless gap. In this case, the extrapolation can cut the axis at a finite photon energy as is observed in some experiments. It is also of interest to differentiate between the two types of Weyl semimetals: those with broken time-reversal symmetry and those with broken spatial-inversion symmetry. We show that, while the former will follow the same behaviour as the 3D Dirac semimetals, for the zero magnetic field properties discussed here, the latter type will show a double step in the optical conductivity at finite doping and a single absorption edge at charge neutrality. The Drude conductivity is always finite in this case, even at charge neutrality.
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