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Register a new userNanoscale Probing of Localized Surface Phonon Polaritons in SiC Nanorods with Swift Electrons
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Surface phonon polaritons hold much potential for subwavelength control and manipulation of light at the infrared to terahertz wavelengths. Here, aided by monochromatic scanning transmission electron microscopy - electron energy loss spectroscopy technique, we study the excitation of optical phonon modes in SiC nanorods. Surface phonon polaritons are modulated by the geometry and size of SiC nanorods. In particular, we study the dispersion relation, spatial dependence and geometry and size effects of surface phonon polaritons. These experimental results are in agreement with dielectric response theory and numerical simulation. Providing critical information for manipulating light in polar dielectrics, these findings should be useful for design of novel nanoscale phonon-photonic devices.
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Surface phonon-polaritons can carry energy on the surface of dielectric films and thus are expected to contribute to heat conduction. However, the contribution of surface phonon-polaritons (SPhPs) to thermal transport has not been experimentally demonstrated yet. In this work, we experimentally measure the effective in-plane thermal conductivity of amorphous silicon nitride membrane and show that it can indeed be increased by SPhPs significantly when the membrane thickness scales down. In particular, by heating up a thin membrane (<100 nm) from 300 to 800 K, the thermal conductivity increases twice due to SPhPs contribution.
Polariton polarization can be described in terms of a pseudospin which can be oriented along the $x,,y,$ or $z$ axis, similarly to electron and hole spin. Unlike electrons and holes where time-reversal symmetry requires that the spin-orbit interaction be odd in the momentum, the analogue of the spin-orbit interaction for polaritons, the so-called TE-TM splitting, is even in the momentum. We calculate and compare spin transport of polariton, electron, and hole systems, in the diffusive regime of many scatterings. After dimensional rescaling diffusive systems with spatially uniform particle densities have identical dynamics, regardless of the particle type. Differences between the three particles appear in spatially non-uniform systems, with pumps at a specific localized point. We consider both oscillating pumps and transient (delta-function) pumps. In such systems each particle type produces distinctive spin patterns. The particles can be distinguished by their differing spatial multipole character, their response and resonances in a perpendicular magnetic field, and their relative magnitude which is largest for electrons and weakest for holes. These patterns are manifested both in response to unpolarized pumps which produce in-plane and perpendicular spin signals, and to polarized pumps where the spin precesses from in-plane to out-of-plane and vice versa. These results will be useful for designing systems with large spin polarization signals, for identifying the dominant spin-orbit interaction and measuring subdominant terms in experimental devices, and for measuring the scattering time and the spin-orbit couplings magnitude.
Long-distance propagation of heat carriers is essential for efficient heat dissipation in microelectronics. However, in dielectric nanomaterials, the primary heat carriers - phonons - can propagate ballistically only for hundreds of nanometres, which limits their heat conduction efficiency. Theory predicts that surface phonon-polaritons (SPhPs) can overcome this limitation and conduct heat without dissipation for hundreds of micrometres. In this work, we experimentally demonstrate such long-distance heat transport by SPhPs. Using the 3$omega$ technique, we measure the in-plane thermal conductivity of SiN nanomembranes for different heater-sensor distances (100 and 200 $mu$m), membrane thicknesses (30 - 200 nm), and temperatures (300 - 400 K). We find that in contrast with thick membranes, thin nanomembranes support heat conduction by SPhPs, as evidenced by an increase in the thermal conductivity with temperature. Remarkably, the thermal conductivity measured 200 $mu$m away from the heater are consistently higher than that measured 100 $mu$m closer. This result suggests that heat conduction by SPhPs is quasi-ballistic over at least hundreds of micrometres. Thus, our findings show that SPhPs can enhance heat dissipation in polar nanomembranes and find applications in thermal management, near-field radiation, and polaritonics.
Imaging materials and inner structures with resolution below the diffraction limit has become of fundamental importance in recent years for a wide variety of applications. In this work, we report sub-diffractive internal structure diagnosis of hexagonal boron nitride by exciting and imaging hyperbolic phonon polaritons. Based on their unique propagation properties, we are able to accurately locate defects in the crystal interior with nanometer resolution. The precise location, size and geometry of the concealed defects is reconstructed by analyzing the polariton wavelength, reflection coefficient and their dispersion. We have also studied the evolution of polariton reflection, transmission and scattering as a function of defect size and photon frequency. The nondestructive high-precision polaritonic structure diagnosis technique introduced here can be also applied to other hyperbolic or waveguide systems, and may be deployed in the next-generation bio-medical imaging, sensing and fine structure analysis.
We report the effects of variation in length on the electronic structure of CdSe nanorods derived from atomic clusters and passivated by fictitious hydrogen atoms. These nanorods are augmented by attaching gold clusters at both the ends to form a nanodumbbell. The goal is to assess the changes at nanolevel after formation of contacts with gold clusters serving as electrodes and compare the results with experimental observations [PRL, 95, 056805 (2005)]. Calculations involving nanorods of length 4.6 Angstrom to 116.6 Angstrom are performed using density functional theory implemented within plane-wave basis set. The binding energy per atom saturates for nanorod of length 116.6 Angstrom. It is interesting to note that upon attaching gold clusters, the nanorods shorter than 27 Angstrom develop metallicity by means of metal induced gap states (MIGS). Longer nanorods exhibit a nanoscale Schottky barrier emerging at the center. For these nanorods, interfacial region closest to the gold electrodes shows a finite density of states in the gap due to MIGS, which gradually decreases towards the center of the nanorod opening up a finite gap. Bader charge analysis indicates localized charge transfer from metal to semiconductor.
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