Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userUncovering Non-Fermi-Liquid Behavior in Hund Metals: Conformal Field Theory Analysis of an SU(2)$times$SU(3) Spin-Orbital Kondo Model
84
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
Hund metals have attracted attention in recent years due to their unconventional superconductivity, which supposedly originates from non-Fermi-liquid (NFL) properties of the normal state. When studying Hund metals using dynamical mean-field theory, one arrives at a self-consistent Hund impurity problem involving a multiorbital quantum impurity with nonzero Hund coupling interacting with a metallic bath. If its spin and orbital degrees of freedom are screened at different energy scales, $T_mathrm{sp} < T_mathrm{orb}$, the intermediate energy window is governed by a novel NFL fixed point, whose nature had not yet been clarified. We resolve this problem by providing an analytical solution of a paradigmatic example of a Hund impurity problem, involving two spin and three orbital degrees of freedom. To this end, we combine a state-of-the-art implementation of the numerical renormalization group, capable of exploiting non-Abelian symmetries, with a generalization of Affleck and Ludwigs conformal field theory (CFT) approach for multichannel Kondo models. We characterize the NFL fixed point of Hund metals in detail for a Kondo model with an impurity forming an SU(2)$times$SU(3) spin-orbital multiplet, tuned such that the NFL energy window is very wide. The impuritys spin and orbital susceptibilities then exhibit striking power-law behavior, which we explain using CFT arguments. We find excellent agreement between CFT predictions and numerical renormalization group results. Our main physical conclusion is that the regime of spin-orbital separation, where orbital degrees of freedom have been screened but spin degrees of freedom have not, features anomalously strong local spin fluctuations: the impurity susceptibility increases as $chi_mathrm{sp}^mathrm{imp} sim omega^{-gamma}$, with $gamma > 1$.
rate research
Read More
We apply conformal field theory analysis to the $k$-channel SU($N$) Kondo system, and find a peculiar behavior in the cases $N > k > 1$, which we call Fermi/non-Fermi mixing: The low temperature scaling is described as the Fermi liquid, while the zero temperature IR fixed point exhibits the non-Fermi liquid signature. We also show that the Wilson ratio is no longer universal for the cases $N > k > 1$. The deviation from the universal value of the Wilson ratio could be used as an experimental signal of the Fermi/non-Fermi mixing.
Orbital differentiation is a common theme in multiorbital systems, yet a complete understanding of it is still missing. Here, we consider a minimal model for orbital differentiation in Hund metals with a highly accurate method: We use the numerical renormalization group as a real-frequency impurity solver for a dynamical mean-field study of three-orbital Hubbard models, where a crystal field shifts one orbital in energy. The individual phases are characterized with dynamic correlation functions and their relation to diverse Kondo temperatures. Upon approaching the orbital-selective Mott transition, we find a strongly suppressed spin coherence scale and uncover the emergence of a singular Fermi liquid and interband doublon-holon excitations. Our theory describes the diverse polarization-driven phenomena in the $t_{2g}$ bands of materials such as ruthenates and iron-based superconductors, and our methodological advances pave the way towards real-frequency analyses of strongly correlated materials.
It was proposed in [(https://doi.org/10.1103/PhysRevLett.114.145301){Chen et al., Phys. Rev. Lett. $mathbf{114}$, 145301 (2015)}] that spin-2 chains display an extended critical phase with enhanced SU$(3)$ symmetry. This hypothesis is highly unexpected for a spin-2 system and, as we argue, would imply an unconventional mechanism for symmetry emergence. Yet, the absence of convenient critical points for renormalization group perturbative expansions, allied with the usual difficulty in the convergence of numerical methods in critical or small-gapped phases, renders the verification of this hypothetical SU$(3)$-symmetric phase a non-trivial matter. By tracing parallels with the well-understood phase diagram of spin-1 chains and searching for signatures robust against finite-size effects, we draw criticism on the existence of this phase. We perform non-Abelian density matrix renormalization group studies of multipolar static correlation function, energy spectrum scaling, single-mode approximation, and entanglement spectrum to shed light on the problem. We determine that the hypothetical SU$(3)$ spin-2 phase is, in fact, dominated by ferro-octupolar correlations and also observe a lack of Luttinger-liquid-like behavior in correlation functions that suggests that is perhaps not critical. We further construct an infinite family of spin-$S$ systems with similar ferro-octupolar-dominated quasi-SU$(3)$-like phenomenology; curiously, we note that the spin-3 version of the problem is located in a subspace of exact G$_2$ symmetry, making this a point of interest for search of Fibonacci topological properties in magnetic systems.
We show how the density-matrix numerical renormalization group (DM-NRG) method can be used in combination with non-Abelian symmetries such as SU(N), where the decomposition of the direct product of two irreducible representations requires the use of a so-called outer multiplicity label. We apply this scheme to the SU(3) symmetrical Anderson model, for which we analyze the finite size spectrum, determine local fermionic, spin, superconducting, and trion spectral functions, and also compute the temperature dependence of the conductance. Our calculations reveal a rich Fermi liquid structure.
We study the Kondo effect in a CNT(left lead)-CNT(QD)-CNT(right lead) structure. Here CNT is a single-wall metallic carbon nanotube, for which 1) the valence and conduction bands of electrons with zero orbital angular momentum ($m=0$) coalesc at the two valley points ${bf{K}}$ and ${bf{K}}$ of the first Brillouin zone and 2) the energy spectrum of electrons with $m e 0$ has a gap whose size is proportional to $|m|$. Following adsorption of hydrogen atoms and application of an appropriately designed gate potential, electron energy levels in the CNT(QD) are tunable to have: 1) two-fold spin degeneracy; 2) two-fold isospin (valley) degeneracy; 3) three-fold orbital degeneracy $m=0,pm1$. As a result, an SU(12) Kondo effect is realized with remarkably high Kondo temperature. Unlike the SU(2) case, the low temperature conductance and magnetic susceptibility have a peak at finite temperature. Moreover, the magnetic susceptibilities for parallel and perpendicular magnetic fields (WRT the tube axis) display anisotropy with a universal ratio $chi_{rm{imp}}^parallel / chi_{rm{imp}}^perp=eta$ that depends only on the electrons orbital and spin $g$ factors.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
