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Register a new userCompeting quasifission and asymmetric fusion-fission in neutron-deficient sub-lead nuclei
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To disentangle the role of shell effects and dynamics, fission fragment mass distributions of $^{191}$Au, a nucleus in the newly identified island of mass asymmetric fission in the sub-lead region, have been measured down to excitation energy of $approx$20 MeV above the fission barrier via two different entrance channels, viz. $^{16}$O+$^{175}$Lu and $^{37}$Cl+$^{154}$Sm reactions. Apart from having signature of the shell effects in both the cases, clear experimental evidence of quasifission has been observed in the mass distributions of the Cl induced reaction, that has also been substantiated by the theoretical calculations. This crucial evidence along with a systematic analysis of available experimental data has revealed that the dynamics in the entrance channel has significant influence on most of the reactions used earlier to explore the persistence of recently discovered mass asymmetry in $beta$-delayed fission at low energy in this mass region, ignoring which might lead to ambiguity in interpreting the heavy-ion data.
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Fragment mass distributions from fission of excited compound nucleus $^{178}$Pt have been deduced from the measured fragment velocities. The $^{178}$Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction $^{36}$Ar + $^{142}$Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of $approx1/3$. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, $A_{L}/A_{H}approx 79/99$, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.
Measurements of mass-angle distributions (MADs) for Cr + W reactions, providing a wide range in the neutron-to-proton ratio of the compound system, (N/Z)CN, have allowed for the dependence of quasifission on the (N/Z)CN to be determined in a model-independent way. Previous experimental and theoretical studies had produced conflicting conclusions. The experimental MADs reveal an increase in contact time and mass evolution of the quasifission fragments with increasing (N/Z)CN, which is indicative of an increase in the fusion probability. The experimental results are in agreement with microscopic time-dependent Hartree-Fock calculations of the quasifission process. The experimental and theoretical results favor the use of the most neutron-rich projectiles and targets for the production of heavy and superheavy nuclei.
Fusion excitation function of $^{35}$Cl + $^{130}$Te system is measured in the energy range around the Coulomb barrier and analyzed in the framework of the coupled-channels approach. The role of projectile deformation, nuclear structure, and the couplings of inelastic excitations and positive Q$-$value neutron transfer channels in sub-barrier fusion are investigated through the comparison of reduced fusion excitation functions of $^{35,37}$Cl +$^{130}$Te systems. The reduced fusion excitation function of $^{35}$Cl + $^{130}$Te system shows substantial enhancement over $^{37}$Cl + $^{130}$Te system in sub-barrier energy region which is attributed to the presence of positive Q-value neutron transfer channels in $^{35}$Cl + $^{130}$Te system. Findings of this work strongly suggest the importance of +2$n$ - transfer coupling in sub-barrier fusion apart from the simple inclusion of inelastic excitations of interacting partners, and are in stark contrast with the results presented by Kohley textit{et al.}, [Phys. Rev. Lett. 107, 202701 (2011)].
Fission of atomic nuclei often produces mass asymmetric fragments. However, the origin of this asymmetry was believed to be different in actinides and in the sub-lead region [A. Andreyev {it et al.}, Phys. Rev. Lett. {bf 105}, 252502 (2010)]. It has recently been argued that quantum shell effects stabilising pear shapes of the fission fragments could explain the observed asymmetries in fission of actinides[G. Scamps and C. Simenel, Nature {bf 564}, 382 (2018)]. This interpretation is tested in the sub-lead region using microscopic mean-field calculations of fission based on the Hartree-Fock approach with BCS pairing correlations. The evolution of the number of protons and neutrons in asymmetric fragments of mercury isotope fissions is interpreted in terms of deformed shell gaps in the fragments. A new method is proposed to investigate the dominant shell effects in the pre-fragments at scission. We conclude that the mechanisms responsible for asymmetric fissions in the sub-lead region are the same as in the actinide region, which is a strong indication of their universality.
The dependence of fusion dynamics on neutron excess for light nuclei is extracted. This is accomplished by comparing the average fusion cross-section at energies just above the fusion barrier for $^{12-15}$C + $^{12}$C with measurements of the interaction cross-section from high evergy collisions. The experimental results indicate that the fusion cross-section associated with dynamics increases with increasing neutron excess. Calculations with a time-dependent Hartree-Fock model fail to describe the observed trend.
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