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Register a new userReduced quasifission competition in fusion reactions forming neutron-rich heavy elements
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Measurements of mass-angle distributions (MADs) for Cr + W reactions, providing a wide range in the neutron-to-proton ratio of the compound system, (N/Z)CN, have allowed for the dependence of quasifission on the (N/Z)CN to be determined in a model-independent way. Previous experimental and theoretical studies had produced conflicting conclusions. The experimental MADs reveal an increase in contact time and mass evolution of the quasifission fragments with increasing (N/Z)CN, which is indicative of an increase in the fusion probability. The experimental results are in agreement with microscopic time-dependent Hartree-Fock calculations of the quasifission process. The experimental and theoretical results favor the use of the most neutron-rich projectiles and targets for the production of heavy and superheavy nuclei.
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To disentangle the role of shell effects and dynamics, fission fragment mass distributions of $^{191}$Au, a nucleus in the newly identified island of mass asymmetric fission in the sub-lead region, have been measured down to excitation energy of $approx$20 MeV above the fission barrier via two different entrance channels, viz. $^{16}$O+$^{175}$Lu and $^{37}$Cl+$^{154}$Sm reactions. Apart from having signature of the shell effects in both the cases, clear experimental evidence of quasifission has been observed in the mass distributions of the Cl induced reaction, that has also been substantiated by the theoretical calculations. This crucial evidence along with a systematic analysis of available experimental data has revealed that the dynamics in the entrance channel has significant influence on most of the reactions used earlier to explore the persistence of recently discovered mass asymmetry in $beta$-delayed fission at low energy in this mass region, ignoring which might lead to ambiguity in interpreting the heavy-ion data.
The angular distributions of fission fragments for the $^{32}$S+$^{184}$W reaction at center-of-mass energies of 118.8, 123.1, 127.3, 131.5, 135.8, 141.1 and 144.4 MeV were measured. The experimental fission excitation function is obtained. The fragment angular anisotropy ($mathcal{A}_{rm exp}$) is found by extrapolating the each fission angular distributions. The measured fission cross sections of the $^{32}$S+$^{182,184}$W reaction are decomposed into fusion-fission, quasifission and fast fission contributions by the dinuclear system model. The total evaporation residue excitation function for the $^{32}$S+$^{184}$W reaction calculated in the framework of the advanced statistical model is in good agreement with the available experimental data up to about $E_{rm c.m.}approx 160$ MeV. The theoretical descriptions of the experimental capture excitation functions for both reactions and quantities $K_0^2$, $<ell^2>$ and $mathcal{A}_{rm exp}$ which characterize angular distributions of the fission products were performed by the same partial capture cross sections at the considered range of beam energy.
The dependence of fusion dynamics on neutron excess for light nuclei is extracted. This is accomplished by comparing the average fusion cross-section at energies just above the fusion barrier for $^{12-15}$C + $^{12}$C with measurements of the interaction cross-section from high evergy collisions. The experimental results indicate that the fusion cross-section associated with dynamics increases with increasing neutron excess. Calculations with a time-dependent Hartree-Fock model fail to describe the observed trend.
Above-barrier fusion cross-sections for an isotopic chain of oxygen isotopes with A=16-19 incident on a $^{12}$C target are presented. Experimental data are compared with both static and dynamical microscopic calculations. These calculations are unable to explain the $sim$37% increase in the average above-barrier fusion cross-section observed for $^{19}$O as compared to $beta$-stable oxygen isotopes. This result suggests that for neutron-rich nuclei existing time-dependent Hartree-Fock calculations underpredict the role of dynamics at near-barrier energies. High-quality measurement of above-barrier fusion for an isotopic chain of increasingly neutron-rich nuclei provides an effective means to probe this fusion dynamics.
The mechanism of fusion hindrance, an effect observed in the reactions of cold, warm and hot fusion leading to production of the superheavy elements, is investigated. A systematics of transfermium production cross sections is used to determine fusion probabilities. Mechanism of fusion hindrance is described as a competition of fusion and quasi-fission. Available evaporation residue cross sections in the superheavy region are reproduced satisfactorily. Analysis of the measured capture cross sections is performed and a sudden disappearance of the capture cross sections is observed at low fusion probabilities. A dependence of the fusion hindrance on the asymmetry of the projectile-target system is investigated using the available data. The most promising pathways for further experiments are suggested.
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