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Register a new userLorentz TEM investigation of chiral spin textures and Neel Skyrmions in asymmetric [Pt/(Co/Ni)$_M$/Ir]$_N$ multi-layer thin films
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We examine magnetic domain patterns in symmetric [Co/Ni]$_M$ and asymmetric [Pt/(Co/Ni)$_M$/Ir]$_N$ multi-layers using Fresnel mode Lorentz transmission electron microscopy (LTEM). In the symmetric multi-layer, where the Dzyaloshinskii-Moriya Interaction is expected to be zero, we observe purely Bloch type domain walls with no preferred chirality. In the asymmetric multi-layers, where significant interfacial DMI is present, we observe domain patterns with chiral Neel domain walls, which evolve into sub-100nm isolated Neel Skyrmions with the application of a perpendicular field. The impact of layer thickness and film stack on interfacial magnetic properties is discussed in the context of developing a tunable multi-layer system for future spintronic applications.
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A combined approach using first-principles calculations and spin dynamics simulations is applied to study Ni/Ir$_{n}$/Pt(111) ($n=0,1,2$) films. The lowest-energy states are predicted to be almost degenerate with negligble energy differences between pure spin-spiral and skyrmionic states. Moreover, for $n=0$ and $n=1$, we found that metastable skyrmioniums can occur, which are characterized by a slightly lower stability with respect to the external fields, enhanced lifetime, and the same critical current density as skyrmions. The spontaneous low temperature skyrmions, with $sim$10 nm to $sim$20 nm size, arise from a large Dzyaloshinskii-Moriya (DM) and Heisenberg exchange interactions ratio and, in particular, from a large in-plane DM vector component for nearest neighbors. The skyrmions become larger, faster and more dispersed with the enhancement of the Ir buffer thickness. Also, with increasing textit{n}, the skyrmions stability decrease when an external magnetic field is applied or the temperature is raised.
Skyrmions are nanoscale spin configurations with topological properties that hold great promise for spintronic devices. Here, we establish their Neel texture, helicity, and size in Ir/Fe/Co/Pt multilayer films by constructing a multipole expansion to model their stray field signatures and applying it to magnetic force microscopy (MFM) images. Furthermore, the demonstrated sensitivity to inhomogeneity in skyrmion properties, coupled with a unique capability to estimate the pinning force governing dynamics, portends broad applicability in the burgeoning field of topological spin textures.
We examine the substructures of magnetic domain walls (DWs) in [Pt/(Co/Ni)$_M$/Ir]$_N$ multi-layers using a combination of micromagnetic theory and Lorentz transmission electron microscopy (LTEM). Thermal stability calculations of Q=$pm$1 substructures (2-$pi$ vertical Bloch lines (VBLs) and DW skyrmions) were performed using a geodesic nudged elastic band (GNEB) model, which supports their metastability at room temperature. Experimental variation in strength of the interfacial Dzyaloshinskii-Moriya interaction (DMI) and film thickness reveals conditions under which these substructures are present and enables the formation of a magnetic phase diagram. Reduced thickness is found to favor Q=$pm$1 substructures likely due to the suppression of hybrid DWs. The results from this study provide an important framework for examining 1-D DW substructures in chiral magnetic materials.
Magnetic skyrmions are nanoscale spin structures recently discovered at room temperature (RT) in multilayer films. Employing their novel topological properties towards exciting technological prospects requires a mechanistic understanding of the excitation and relaxation mechanisms governing their stability and dynamics. Here we report on the magnetization dynamics of RT Neel skyrmions in Ir/Fe/Co/Pt multilayer films. We observe a ubiquitous excitation mode in the microwave absorption spectrum, arising from the gyrotropic resonance of topological skyrmions, and robust over a wide range of temperatures and sample compositions. A combination of simulations and analytical calculations establish that the spectrum is shaped by the interplay of interlayer and interfacial magnetic interactions unique to multilayers, yielding skyrmion resonances strongly renormalized to lower frequencies. Our work provides fundamental spectroscopic insights on the spatiotemporal dynamics of topological spin structures, and crucial directions towards their functionalization in nanoscale devices.
We characterize asymmetric growth of magnetic bubble domains in perpendicularly magnetized Co/Ni multi-layers grown on Pt$_x$Ir$_{1-x}$ seedlayers by application of perpendicular and in-plane magnetic fields. Using a refined model of domain wall creep that incorporates contributions from the anisotropic elastic energy, $varepsilon$, and a chirality-dependent prefactor, $v_0$, we elucidate factors that govern the mobility of Dzyaloshinskii domain walls as a function of seedlayer composition. The interfacial Dzyaloshinskii-Moriya Interaction magnitude is found to decrease monotonically with $x_{Ir}$, which is independently confirmed by Brillouin light scattering (BLS). Moreover, the persistence of significant asymmetry in velocity curves across the full composition range supports previous assertions that a chirality-dependent attempt frequency akin to chiral damping could play a critical role in the observed trends. This work helps resolve fundamental questions about the factors governing Dzyaloshinskii DW creep and demonstrates varying Pt-Ir seedlayer composition as a method to tune DMI.
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