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Disentangling factors governing Dzyaloshinskii domain wall creep in Co/Ni thin films using Pt$_x$Ir$_{1-x}$ seedlayers

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 Added by Vincent Sokalski
 Publication date 2018
  fields Physics
and research's language is English




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We characterize asymmetric growth of magnetic bubble domains in perpendicularly magnetized Co/Ni multi-layers grown on Pt$_x$Ir$_{1-x}$ seedlayers by application of perpendicular and in-plane magnetic fields. Using a refined model of domain wall creep that incorporates contributions from the anisotropic elastic energy, $varepsilon$, and a chirality-dependent prefactor, $v_0$, we elucidate factors that govern the mobility of Dzyaloshinskii domain walls as a function of seedlayer composition. The interfacial Dzyaloshinskii-Moriya Interaction magnitude is found to decrease monotonically with $x_{Ir}$, which is independently confirmed by Brillouin light scattering (BLS). Moreover, the persistence of significant asymmetry in velocity curves across the full composition range supports previous assertions that a chirality-dependent attempt frequency akin to chiral damping could play a critical role in the observed trends. This work helps resolve fundamental questions about the factors governing Dzyaloshinskii DW creep and demonstrates varying Pt-Ir seedlayer composition as a method to tune DMI.

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We study the magnetic properties of perpendicularly magnetised Pt/Co/Ir thin films and investigate the domain wall creep method of determining the interfacial Dzyaloshinskii-Moriya (DM) interaction in ultra-thin films. Measurements of the Co layer thickness dependence of saturation magnetisation, perpendicular magnetic anisotropy, and symmetric and antisymmetric (i.e. DM) exchange energies in Pt/Co/Ir thin films have been made to determine the relationship between these properties. We discuss the measurement of the DM interaction by the expansion of a reverse domain in the domain wall creep regime. We show how the creep parameters behave as a function of in-plane bias field and discuss the effects of domain wall roughness on the measurement of the DM interaction by domain expansion. Whereas modifications to the creep law with DM field and in-plane bias fields have taken into account changes in the energy barrier scaling parameter $alpha$, we find that both $alpha$ and the velocity scaling parameter $v_{0}$ change as a function of in-plane bias field.
We examine the substructures of magnetic domain walls (DWs) in [Pt/(Co/Ni)$_M$/Ir]$_N$ multi-layers using a combination of micromagnetic theory and Lorentz transmission electron microscopy (LTEM). Thermal stability calculations of Q=$pm$1 substructures (2-$pi$ vertical Bloch lines (VBLs) and DW skyrmions) were performed using a geodesic nudged elastic band (GNEB) model, which supports their metastability at room temperature. Experimental variation in strength of the interfacial Dzyaloshinskii-Moriya interaction (DMI) and film thickness reveals conditions under which these substructures are present and enables the formation of a magnetic phase diagram. Reduced thickness is found to favor Q=$pm$1 substructures likely due to the suppression of hybrid DWs. The results from this study provide an important framework for examining 1-D DW substructures in chiral magnetic materials.
We report on magnetic domain wall velocity measurements in ultrathin Pt/Co(0.5-0.8 nm)/Pt films with perpendicular anisotropy over a large range of applied magnetic fields. The complete velocity-field characteristics are obtained, enabling an examination of the transition between thermally activated creep and viscous flow: motion regimes predicted from general theories for driven elastic interfaces in weakly disordered media. The dissipation limited flow regime is found to be consistent with precessional domain wall motion, analysis of which yields values for the damping parameter, $alpha$.
We studied electric field modification of magnetic properties in a Pt/Co/AlO$_x$ trilayer via magneto-optical Kerr microscopy. We observed the spontaneous formation of labyrinthine magnetic domain structure due to thermally activated domain nucleation and propagation under zero applied magnetic field. A variation of the period of the labyrinthine structure under electric field is observed as well as saturation magnetization and magnetic anisotropy variations. Using an analytical formula of the stripe equilibrium width we estimate the variation of the interfacial Dzyaloshinskii-Moriya interaction under electric field as function of the exchange stiffness constant.
We have characterized the strength of the interfacial Dyzaloshinskii-Moriya interaction (DMI) in ultrathin perpendicularly magnetized CoFeB/MgO films, grown on different underlayers of W, TaN, and Hf, using two experimental methods. First, we determined the effective DMI field from measurements of field-driven domain wall motion in the creep regime, where applied in-plane magnetic fields induce an anisotropy in the wall propagation that is correlated with the DMI strength. Second, Brillouin light spectroscopy was employed to quantify the frequency non-reciprocity of spin waves in the CoFeB layers, which yielded an independent measurement of the DMI. By combining these results, we show that DMI estimates from the different techniques only yield qualitative agreement, which suggests that open questions remain on the underlying models used to interpret these results.
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