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The time-dependent transition between a diabatic interaction potential in the entrance channel and an adiabatic potential during the fusion process is investigated within the two-center shell model. A large hindrance is obtained for the motion to smaller elongations of near symmetric dinuclear systems. The comparison of the calculated energy thresholds for the complete fusion in different relevant collective variables shows that the dinuclear system prefers to evolve in the mass asymmetry coordinate by nucleon transfer to the compound nucleus.
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Within the dinuclear system (DNS) conception, instead of solving Fokker-Planck Equation (FPE) analytically, the Master equation is solved numerically to calculate the fusion probability of super-heavy nuclei, so that the harmonic oscillator approximation to the potential energy of the DNS is avoided. The relative motion concerning the energy, the angular momentum, and the fragment deformation relaxations is explicitly treated to couple with the diffusion process, so that the nucleon transition probabilities, which are derived microscopically, are time-dependent. Comparing with the analytical solution of FPE, our results preserve more dynamical effects. The calculated evaporation residue cross sections for one-neutron emission channel of Pb-based reactions are basically in agreement with the known experimental data within one order of magnitude.
The dependence of fusion cross section on the isotopic composition of colliding nuclei is analysed within the dinuclear system concept for compound nucleus formation. Probabilities of fusion and surviving probabilities, ingredients of the evaporation residue cross sections, depend decisively on the neutron numbers of the dinuclear system. Evaporation residue cross sections for the production of actinides and superheavy nuclei, listed in table form, are discussed and compared with existing experimental data. Neutron-rich radioactive projectiles are shown to lead to similar fusion cross sections as stable projectiles.
Within the framework of the dinuclear system model, the production mechanism of neutron-rich heavy nuclei around N = 162 has been investigated systematically. The isotopic yields in the multinucleon transfer reaction of $^{238}$U + $^{248}$Cm was analyzed and compared the available experimental data. Systematics on the production of superheavy nuclei via $^{238}$U on $^{252,254}$Cf, $^{254}$Es and $^{257}$Fm is investigated. It is found that the shell effect is of importance in the formation of neutron-rich nuclei around N=162 owing to the enhancement of fission barrier. The fragments in the multinucleon transfer reactions manifest the broad isotopic distribution and are dependent on the beam energy. The polar angles of the fragments tend to the forward emission with increasing the beam energy. The production cross sections of new isotopes are estimated and heavier targets are available for the neutron-rich superheavy nucleus formation. The optimal system and beam energy are proposed for the future experimental measurements.
The heavy-ion fusion reactions induced by neutron-rich nuclei are investigated with the improved quantum molecular dynamics (ImQMD) model. With a subtle consideration of the neutron skin thickness of nuclei and the symmetry potential, the stability of nuclei and the fusion excitation functions of heavy-ion fusion reactions $^{16}$O+$^{76}$Ge, $^{16}$O+$^{154}$Sm, $^{40}$Ca+$^{96}$Zr and $^{132}$Sn+$^{40}$Ca are systematically studied. The fusion cross sections of these reactions at energies around the Coulomb barrier can be well reproduced by using the ImQMD model. The corresponding slope parameter of the symmetry energy adopted in the calculations is $L approx 78$ MeV and the surface energy coefficient is $g_{rm sur}=18pm 1.5$ MeVfm$^2$. In addition, it is found that the surface-symmetry term significantly influences the fusion cross sections of neutron-rich fusion systems. For sub-barrier fusion, the dynamical fluctuations in the densities of the reaction partners and the enhanced surface diffuseness at neck side result in the lowering of the fusion barrier.
Nucleon-transfer sum rules have been assessed via a consistent reanalysis of cross-section data from neutron-adding ($d$,$p$) and -removing ($d$,$t$) reactions on well-deformed isotopes of Gd, Dy, Er, Yb, and W, with $92leq Nleq108$, studied at the Niels Bohr Institute in the 1960s and 1970s. These are complemented by new measurements of cross sections using the ($d$,$p$), ($d$,$t$), and ($p$,$d$) reactions on a subset of these nuclei. The sum rules, defined in a Nilsson-model framework, are remarkably consistent. A single overall normalization is used in the analysis, which appears to be sensitive to assumptions about the reaction mechanism, and in the case of sums using the ($d$,$t$) reaction, differs from values determined from reactions on spherical systems.
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