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Particle transfer and fusion cross-section for Super-heavy nuclei in dinuclear system

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 Added by Qingfeng Li
 Publication date 2005
  fields
and research's language is English




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Within the dinuclear system (DNS) conception, instead of solving Fokker-Planck Equation (FPE) analytically, the Master equation is solved numerically to calculate the fusion probability of super-heavy nuclei, so that the harmonic oscillator approximation to the potential energy of the DNS is avoided. The relative motion concerning the energy, the angular momentum, and the fragment deformation relaxations is explicitly treated to couple with the diffusion process, so that the nucleon transition probabilities, which are derived microscopically, are time-dependent. Comparing with the analytical solution of FPE, our results preserve more dynamical effects. The calculated evaporation residue cross sections for one-neutron emission channel of Pb-based reactions are basically in agreement with the known experimental data within one order of magnitude.

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The time-dependent transition between a diabatic interaction potential in the entrance channel and an adiabatic potential during the fusion process is investigated within the two-center shell model. A large hindrance is obtained for the motion to smaller elongations of near symmetric dinuclear systems. The comparison of the calculated energy thresholds for the complete fusion in different relevant collective variables shows that the dinuclear system prefers to evolve in the mass asymmetry coordinate by nucleon transfer to the compound nucleus.
The dependence of fusion cross section on the isotopic composition of colliding nuclei is analysed within the dinuclear system concept for compound nucleus formation. Probabilities of fusion and surviving probabilities, ingredients of the evaporation residue cross sections, depend decisively on the neutron numbers of the dinuclear system. Evaporation residue cross sections for the production of actinides and superheavy nuclei, listed in table form, are discussed and compared with existing experimental data. Neutron-rich radioactive projectiles are shown to lead to similar fusion cross sections as stable projectiles.
A variety of phenomena connected with the formation of a dinuclear complex is observed in the heavy ion collisions at low energies. The dinuclear system model allows us to analyze the experimental data and to interpret them by comparison of the partial capture, fusion and evaporation residue cross sections measured for the different reactions leading to the same compound nucleus. The comparison of theoretical and experimental values of the mass and angular distributions of the reaction products gives us a detailed information about reaction mechanism forming the observed yields. The observed very small cross sections of the evaporation residues may be explained by the strong fusion hindrance and/or instability of the heated and rotating compound nucleus and smallness of its survival probability. The fusion hindrance arises due to competition between complete fusion and quasifission while the smallness of survival probability is connected with the decrease of the fission barrier at large excitation energy and angular momentum of compound nucleus.
The synthesis of superheavy elements is analysed within the dinuclear system concept of compound nucleus formation. The perspectives for using radioactive beams in complete fusion reactions are discussed.
Potential energies, moments of inertia, quadrupole and octupole moments of dinuclear systems are compared with the corresponding quantities of strongly deformed nuclei. As dinuclear system we denote two touching nuclei (clusters). It is found that the hyperdeformed states of nuclei are close to those of nearly symmetric dinuclear systems, whereas the superdeformed states are considered as states of asymmetric dinuclear systems. The superdeformed and hyperdeformed states constructed from two touching clusters have large octupole deformations. The experimental measurement of octupole deformation of the highly deformed nuclei can answer whether these nuclei have cluster configurations as described by the dinuclear model.
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