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Excitation of molecules by incident incoherent electromagnetic radiation, such as sunlight, is described in detail and contrasted with the effect of coherent (e.g. laser) light. The nature of the quantum coherences induced by the former, relevant to transport processes in nature and in technology, is emphasized. Both equilibrium and steady state scenarios are discussed, Three examples: simple models, calcium excitation in polarized light, and the isomerization of retinal in rhodopsin are used to expose the underlying qualitative nature of the established coherences.
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We investigate theoretically the effects of vacuum-induced coherence (VIC) on magneto-optical rotation (MOR). We carry out a model study to show that VIC in the presence of a control laser and a magnetic field can lead to large enhancement in the rotation of the plane of polarization of a linearly polarized weak laser with vanishing circular dichroism. This effect can be realized in cold molecular gases and may be used as a sensitive probe for VIC. Such a large MOR angle can also be used to detect weak magnetic field with large measurement sensitivity.
We demonstrate theoretically the noise-stimulated enhancement of quantum coherence in a superconducting flux qubit. First, an external classical noise can increase the off-diagonal components of the qubit density matrix. Second, in the presence of noise, the Rabi oscillations survive for times significantly longer than the Rabi decay time in a noiseless system. These Rabi oscillations appear as a modulation of the forced response of the qubit to the ac driving field. These effects can be considered as a manifestation of quantum stochastic resonance and are relevant to experimental techniques, such as Rabi spectroscopy.
We demonstrate a different scheme to perform optical sectioning of a sample based on the concept of induced coherence [Zou et al., Phys. Rev. Lett. 67, 318 (1991)]. This can be viewed as a different type of optical coherence tomography scheme where the varying reflectivity of the sample along the direction of propagation of an optical beam translates into changes of the degree of first-order coherence between two beams. As a practical advantage the scheme allows probing the sample with one wavelength and measuring photons with another wavelength. In a bio-imaging scenario, this would result in a deeper penetration into the sample because of probing with longer wavelengths, while still using the optimum wavelength for detection. The scheme proposed here could achieve submicron axial resolution by making use of nonlinear parametric sources with broad spectral bandwidth emission.
We introduce and theoretically demonstrate a quantum metamaterial made of dense ultracold neutral atoms loaded into an inherently defect-free artificial crystal of light, immune to well-known critical chal- lenges inevitable in conventional solid-state platforms. We demonstrate an all-optical control on ultrafast time scales over the photonic topological transition of the isofrequency contour from an open to close topology at the same frequency. This atomic lattice quantum metamaterial enables a dynamic manipula- tion of the decay rate of a probe quantum emitter by more than an order of magnitude. This proposal may lead to practically lossless, tunable and topologically-reconfigurable quantum metamaterials, for single- or few-photon-level applications as varied as quantum sensing, quantum information processing, and quantum simulations using metamaterials.
We observe the quantum coherent dynamics of atomic spinor wavepackets in the double well potentials of a far-off-resonance optical lattice. With appropriate initial conditions the system Rabi oscillates between the left and right localized states of the ground doublet, and at certain times the wavepacket corresponds to a coherent superposition of these mesoscopically distinguishable quantum states. The atom/optical double well potential is a flexible and powerful system for further study of mesoscopic quantum coherence, quantum control and the quantum/classical transition.
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