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Probing vacuum-induced coherence via magneto-optical rotation in molecular systems

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 Added by Pardeep Kumar
 Publication date 2015
  fields Physics
and research's language is English




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We investigate theoretically the effects of vacuum-induced coherence (VIC) on magneto-optical rotation (MOR). We carry out a model study to show that VIC in the presence of a control laser and a magnetic field can lead to large enhancement in the rotation of the plane of polarization of a linearly polarized weak laser with vanishing circular dichroism. This effect can be realized in cold molecular gases and may be used as a sensitive probe for VIC. Such a large MOR angle can also be used to detect weak magnetic field with large measurement sensitivity.



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121 - A. Vafafard , S. Hughes , 2017
Vacuum induced coherence in a strongly coupled cavity consisting of a three-level system is studied theoretically. The effects of the strong coupling to electromagnetic field vacuum are examined by solution of an open-system quantum master equation. The numerical results show that the system exhibits population trapping, and the numerical results are interpreted with analytical expressions derived from a new basis in the weak excitation regime. We further show that the generated effects can be probed with weak external fields. Moreover, it is shown that the induced coherence can be controlled by the applied field parameters like field detuning. Finally, we study the trapping dynamics in the strong field excitation regime, and also demonstrate that a recently proposed asymmetric pumping regime (limited to the weak coupling regime) can remove the radiative decay of coherent Rabi oscillations, with both weak and strong excitation fields.
We predict theoretically and demonstrate experimentally an ellipticity-dependent nonlinear magneto-optic rotation of elliptically-polarized light propagating in a coherent atomic medium. We show that this effect results from a hexadecapole and higher order momenta of atomic coherence, and is associated with an enhancement of Kerr and higher orders nonlinearities accompanied by suppression of the other linear and nonlinear susceptibility terms of the medium. These nonlinearities might be useful for quantum signal processing. In particular, we report an observation of an enhancement the polarization rotation of elliptically polarized light resonant with the 5S_{1/2} F=2 -> 5P_{1/2} F=1 transition of Rb87.
140 - Amro Dodin , Paul Brumer 2021
Excitation of molecules by incident incoherent electromagnetic radiation, such as sunlight, is described in detail and contrasted with the effect of coherent (e.g. laser) light. The nature of the quantum coherences induced by the former, relevant to transport processes in nature and in technology, is emphasized. Both equilibrium and steady state scenarios are discussed, Three examples: simple models, calcium excitation in polarized light, and the isomerization of retinal in rhodopsin are used to expose the underlying qualitative nature of the established coherences.
We have studied the intensity correlations between two orthogonally linearly polarized components of a laser field propagating through a resonant atomic medium. These experiments have been performed in a Rubidium atomic vapor. We observe that the correlations between the orthogonally polarized components of the laser beam are maximal in the absence of a magnetic field. The magnitude of the correlations depends on the applied magnetic field, and the magnitude first decreases and then increases with increasing magnetic field. Minimal correlations and maximal rotation angles are observed at the same magnetic fields. The width of the correlation function is directly proportional to the excited state lifetime and inversely proportional to the Rabi frequency of laser field. These results can be useful for improving optical magnetometers and for optical field or atomic spin squeezing.
86 - A.B. Matsko 2001
When linearly polarized light propagates through a medium in which elliptically polarized light would undergo self-rotation, squeezed vacuum can appear in the orthogonal polarization. A simple relationship between self-rotation and the degree of vacuum squeezing is developed. Taking into account absorption, we find the optimum conditions for squeezing in any medium that can produce self-rotation. We then find analytic expressions for the amount of vacuum squeezing produced by an atomic vapor when light is near-resonant with a transition between various low-angular-momentum states. Finally, we consider a gas of multi-level Rb atoms, and analyze squeezing for light tuned near the D-lines under realistic conditions.
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