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Effect of hyperfine structure on atomic frequency combs in Pr:YSO

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 Added by Aditya Sharma
 Publication date 2020
  fields Physics
and research's language is English




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Quantum memory will be a key component in future quantum networks, and atomic frequency combs (AFCs) in rare-earth-doped crystals are one promising platform for realizing this technology. We theoretically and experimentally investigate the formation of AFCs in Pr3+:Y2SiO5, with an overall bandwidth of 120 MHz and tooth spacing ranging from 0.1 MHz to 20 MHz, showing agreement between our calculations and measurements. We observe that the echo efficiency depends crucially on the AFC tooth spacing. Our results suggest approaches to developing a high-efficiency AFC quantum memory.

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We propose a Raman quantum memory scheme that uses several atomic ensembles to store and retrieve the multimode highly entangled state of an optical quantum frequency comb, such as the one produced by parametric down-conversion of a pump frequency comb. We analyse the efficiency and the fidelity of such a quantum memory. Results show that our proposal may be helpful to multimode information processing using the different frequency bands of an optical frequency comb.
We demonstrate ultrafast coherent coupling between an atomic qubit stored in a single trapped cadmium ion and a photonic qubit represented by two resolved frequencies of a photon. Such ultrafast coupling is crucial for entangling networks of remotely-located trapped ions through photon interference, and is also a key component for realizing ultrafast quantum gates between Coulomb-coupled ions.
We have developed the full theory of a synchronously pumped type I optical parametric oscillator (SPOPO). We derive expressions for the oscillation threshold and the characteristics of the generated mode-locked signal beam. We calculate the output quantum fluctuations of the device, and find that, in the degenerate case (coincident signal and idler set of frequencies), perfect squeezing is obtained when one approaches threshold from below for a well defined super-mode, or frequency comb, consisting of a coherent linear superposition of signal modes of different frequencies which are resonant in the cavity.
The magnetic hyperfine structure constants have been calculated for low-lying levels in neutral gold atom and gold-like ion of mercury taking into account Bohr--Weisskopf (BW) effect. BW effect is represented as a product of atomic and nuclear ($d_mathrm{nuc}$) factors. We have calculated the atomic factors, which enable one to extract BW-correction values for far from stability gold nuclei from the experimental data. The possible uncertainty of our atomic calculations have been estimated by the comparison with the available experimental data. It has been shown that the standard single-particle approach in $d_mathrm{nuc}$ calculation reasonably well describes experimental data for $11/2^-$ gold isomers and $3/2^+$ ground state of $rm ^{199}Au$. At the same time, it fails to describe the hyperfine constant in $^{197}mathrm{Au}$. This indicates the more pronounced configuration mixing in $rm ^{197}Au$ than in $rm ^{199}Au$.
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