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Register a new userMeasurement of the Background Activities of a 100Mo-enriched powder sample for AMoRE crystal material using a single high purity germanium detector
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The Advanced Molybdenum-based Rare process Experiment (AMoRE) searches for neutrino-less double-beta (0{ u}b{eta}b{eta}) decay of 100Mo in enriched molybdate crystals. The AMoRE crystals must have low levels of radioactive contamination to achieve low background signals with energies near the Q-value of the 100Mo 0{ u}b{eta}b{eta} decay. To produce low-activity crystals, radioactive contaminants in the raw materials used to form the crystals must be controlled and quantified. 100EnrMoO3 powder, which is enriched in the 100Mo isotope, is of particular interest as it is the source of 100Mo in the crystals. A high-purity germanium detector having 100% relative efficiency, named CC1, is being operated in the Yangyang underground laboratory. Using CC1, we collected a gamma spectrum from a 1.6-kg 100EnrMoO3 powder sample enriched to 96.4% in 100Mo. Activities were analyzed for the isotopes 228Ac, 228Th, 226Ra, and 40K. They are long-lived naturally occurring isotopes that can produce background signals in the region of interest for AMoRE. Activities of both 228Ac and 228Th were < 1.0 mBq/kg at 90% confidence level (C.L.). The activity of 226Ra was measured to be 5.1 pm 0.4 (stat) pm 2.2 (syst) mBq/kg. The 40K activity was found as < 16.4 mBq/kg at 90% C.L.
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The Advanced Molybdenum-based Rare process Experiment in its second phase (AMoRE-II) will search for neutrinoless double-beta (0{ u}b{eta}b{eta}) decay of 100Mo in 200 kg of molybdate crystals. To achieve the zero-background level in the energy range of the double-beta decay Q-value of 100Mo, the radioactive contamination levels in AMoRE crystals should be low. 100EnrMoO3 powder, which is enriched in the 100Mo isotope, is used to grow the AMoRE crystals. A shielded array of fourteen high-purity germanium detectors with 70% relative efficiency each was used for the measurement of background activities in a sample of 9.6-kg powder. The detector system named CAGe located at the Yangyang underground laboratory was designed for measuring low levels of radioactivity from natural radioisotopes or cosmogenic nuclides such as 228Ac, 228Th, 226Ra, 88Y, and 40K. The activities of 228Ac and 228Th in the powder sample were 0.88 pm 0.12 mBq/kg and 0.669 pm 0.087 mBq/kg, respectively. The activity of 226Ra was measured to be 1.50 pm 0.23 mBq/kg. The activity of 88Y was 0.101 pm 0.016 mBq/kg. The activity of 40K was found as 36.0 pm 4.1 mBq/kg.
The AMoRE is an experiment to search for neutrinoless double-beta decay of 100Mo in molybdate crystal scintillators using a cryogenic detection technique. The crystals are equipped with metallic magnetic calorimeter sensors that detect both phonon and photon signals at temperatures of a few tens of mK. Simultaneous measurements of thermal and scintillation signals produced by particle interactions in the crystals by MMC sensors provide high energy resolution and efficient particle discrimination. AMoRE-Pilot, an R&D phase with six 48deplCa100MoO4 crystals and a total mass of ~1.9 kg in the final configuration, operated at the 700 m deep Yangyang underground laboratory (Y2L). After completion of the AMoRE-Pilot run at the end of 2018, AMoRE-I with a ~6 kg crystal array comprised of thirteen 48deplCa100MoO4 and five Li2100MoO4 crystals is currently being assembled and installed at Y2L. We have secured 110 kg of 100Mo-isotope-enriched MoO3 powder for the production of crystals for the AMoRE-II phase, which will have ~200 kg of molybdate crystals and operate at Yemilab, a new underground laboratory located ~1,100 m deep in the Handeok iron mine that is currently being excavated and with a scheduled completion date of December 2020. AMoRE-II is expected to improve the upper limit on the effective Majorana neutrino mass to cover the entire inverted hierarchy neutrino mass region: 20-50 meV, in the case when no such decays are observed. Results from AMoRE-Pilot and progress of the preparations for AMoRE-I and AMoRE-II are presented.
A high-purity co-axial germanium detector has been calibrated in efficiency to a precision of about 0.15% over a wide energy range. High-precision scans of the detector crystal and gamma-ray source measurements have been compared to Monte-Carlo simulations to adjust the dimensions of a detector model. For this purpose, standard calibration sources and short-lived on-line sources have been used. The resulting efficiency calibration reaches the precision needed e.g. for branching ratio measurements of super-allowed beta decays for tests of the weak-interaction standard model.
We have studied channeling effects in a Cesium Iodide (CsI) crystal that is similar in composition to the ones being used in a search for Weakly Interacting Massive Particles (WIMPs) dark matter candidates, and measured its energy-dependent quenching factor, the relative scintillation yield for electron and nuclear recoils. The experimental results are reproduced with a GEANT4 simulation that includes a model of the scintillation efficiency as a function of electronic stopping power. We present the measured and simulated quenching factors and the estimated effects of channeling.
Following work done in the energy region above 100 keV, the high-precision calibration of a co-axial high-purity germanium detector has been continued in the energy region below 100 keV. Previous measurements or Monte-Carlo simulations have been repeated with higher statistics and new source measurements have been added. A precision as in the high-energy part, i.e. an absolute precision for the detection efficiency of 0.2%, has been reached. The low-energy behaviour of the germanium detector was further scrutinized by studying the germanium X-ray escape probability for the detection of low-energy photons. In addition, one experimental point, a gamma ray at 2168 keV from the decay of 38K, has been included for the total-to-peak ratios agreeing well with simulations. The same gamma ray was also added for the single- and double-escape probabilities. Finally, the long term stability of the efficiency of the germanium detector was investigated by regularly measuring the full-energy peak efficiency with a precisely calibrated 60Co source and found to be perfectly stable over a period of 10 years.
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