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Register a new userMeasurement of the Background Activities of a 100Mo-enriched Powder Sample for an AMoRE Crystal Material by using Fourteen High-Purity Germanium Detectors
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The Advanced Molybdenum-based Rare process Experiment in its second phase (AMoRE-II) will search for neutrinoless double-beta (0{ u}b{eta}b{eta}) decay of 100Mo in 200 kg of molybdate crystals. To achieve the zero-background level in the energy range of the double-beta decay Q-value of 100Mo, the radioactive contamination levels in AMoRE crystals should be low. 100EnrMoO3 powder, which is enriched in the 100Mo isotope, is used to grow the AMoRE crystals. A shielded array of fourteen high-purity germanium detectors with 70% relative efficiency each was used for the measurement of background activities in a sample of 9.6-kg powder. The detector system named CAGe located at the Yangyang underground laboratory was designed for measuring low levels of radioactivity from natural radioisotopes or cosmogenic nuclides such as 228Ac, 228Th, 226Ra, 88Y, and 40K. The activities of 228Ac and 228Th in the powder sample were 0.88 pm 0.12 mBq/kg and 0.669 pm 0.087 mBq/kg, respectively. The activity of 226Ra was measured to be 1.50 pm 0.23 mBq/kg. The activity of 88Y was 0.101 pm 0.016 mBq/kg. The activity of 40K was found as 36.0 pm 4.1 mBq/kg.
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The Advanced Molybdenum-based Rare process Experiment (AMoRE) searches for neutrino-less double-beta (0{ u}b{eta}b{eta}) decay of 100Mo in enriched molybdate crystals. The AMoRE crystals must have low levels of radioactive contamination to achieve low background signals with energies near the Q-value of the 100Mo 0{ u}b{eta}b{eta} decay. To produce low-activity crystals, radioactive contaminants in the raw materials used to form the crystals must be controlled and quantified. 100EnrMoO3 powder, which is enriched in the 100Mo isotope, is of particular interest as it is the source of 100Mo in the crystals. A high-purity germanium detector having 100% relative efficiency, named CC1, is being operated in the Yangyang underground laboratory. Using CC1, we collected a gamma spectrum from a 1.6-kg 100EnrMoO3 powder sample enriched to 96.4% in 100Mo. Activities were analyzed for the isotopes 228Ac, 228Th, 226Ra, and 40K. They are long-lived naturally occurring isotopes that can produce background signals in the region of interest for AMoRE. Activities of both 228Ac and 228Th were < 1.0 mBq/kg at 90% confidence level (C.L.). The activity of 226Ra was measured to be 5.1 pm 0.4 (stat) pm 2.2 (syst) mBq/kg. The 40K activity was found as < 16.4 mBq/kg at 90% C.L.
The AMoRE is an experiment to search for neutrinoless double-beta decay of 100Mo in molybdate crystal scintillators using a cryogenic detection technique. The crystals are equipped with metallic magnetic calorimeter sensors that detect both phonon and photon signals at temperatures of a few tens of mK. Simultaneous measurements of thermal and scintillation signals produced by particle interactions in the crystals by MMC sensors provide high energy resolution and efficient particle discrimination. AMoRE-Pilot, an R&D phase with six 48deplCa100MoO4 crystals and a total mass of ~1.9 kg in the final configuration, operated at the 700 m deep Yangyang underground laboratory (Y2L). After completion of the AMoRE-Pilot run at the end of 2018, AMoRE-I with a ~6 kg crystal array comprised of thirteen 48deplCa100MoO4 and five Li2100MoO4 crystals is currently being assembled and installed at Y2L. We have secured 110 kg of 100Mo-isotope-enriched MoO3 powder for the production of crystals for the AMoRE-II phase, which will have ~200 kg of molybdate crystals and operate at Yemilab, a new underground laboratory located ~1,100 m deep in the Handeok iron mine that is currently being excavated and with a scheduled completion date of December 2020. AMoRE-II is expected to improve the upper limit on the effective Majorana neutrino mass to cover the entire inverted hierarchy neutrino mass region: 20-50 meV, in the case when no such decays are observed. Results from AMoRE-Pilot and progress of the preparations for AMoRE-I and AMoRE-II are presented.
A study of signals originating near the lithium-diffused n+ contact of p-type point contact (PPC) high purity germanium detectors (HPGe) is presented. The transition region between the active germanium and the fully dead layer of the n+ contact is examined. Energy depositions in this transition region are shown to result in partial charge collection. This provides a mechanism for events with a well defined energy to contribute to the continuum of the energy spectrum at lower energies. A novel technique to quantify the contribution from this source of background is introduced. Experiments that operate germanium detectors with a very low energy threshold may benefit from the methods presented herein.
The GERmanium Detector Array, GERDA, will search for neutrinoless double beta decay in 76Ge at the National Gran Sasso Laboratory of the INFN. Bare high-purity germanium detectors enriched in 76Ge will be submerged in liquid argon serving simultaneously as a shield against external radioactivity and as a cooling medium. In GERDA Phase-I, reprocessed enriched-Ge detectors, which were previously operated by the Heidelberg-Moscow and IGEX collaborations, will be redeployed. Before operating the enriched detectors, tests are performed with non-enriched bare HPGe detectors in the GERDA underground Detector Laboratory to test the Phase-I detector assembly, the detector handling protocols, the refurbishment technology and to study the long-term stability in liquid argon. The leakage currents in liquid argon and liquid nitrogen have been extensively studied under varying gamma irradiation conditions. In total three non-enriched high-purity p-type prototype germanium detectors have been operated successfully. The detector performance is stable over the long-term measurements. For the first time, performance of bare high-purity germanium detectors in liquid argon is reported.
Large, high-purity, germanium (HPGe) detectors are needed for neutrinoless double-beta decay and dark matter experiments. Currently, large (> 4 inches in diameter) HPGe crystals can be grown at the University of South Dakota (USD). We verify that the quality of the grown crystals is sufficient for use in large detectors by fabricating and characterizing smaller HPGe detectors made from those crystals. We report the results from eight detectors fabricated over six months using crystals grown at USD. Amorphous germanium (a-Ge) contacts are used for blocking both electrons and holes. Two types of geometry were used to fabricate HPGe detectors. As a result, the fabrication process of small planar detectors at USD is discussed in great detail. The impact of the procedure and geometry on the detector performance was analyzed for eight detectors. We characterized the detectors by measuring the leakage current, capacitance, and energy resolution at 662 keV with a Cs-137 source. Four detectors show good performance, which indicates that crystals grown at USD are suitable for making HPGe detectors.
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