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Register a new userSpin-orbit torques in a Rashba honeycomb antiferromagnet
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Recent experiments on switching antiferromagnetic domains by electric current pulses have attracted a lot of attention to spin-orbit torques in antiferromagnets. In this work, we employ the tight-binding model solver, kwant, to compute spin-orbit torques in a two-dimensional antiferromagnet on a honeycomb lattice with strong spin-orbit interaction of Rashba type. Our model combines spin-orbit interaction, local s-d-like exchange, and scattering of conduction electrons on on-site disorder potential to provide a microscopic mechanism for angular momentum relaxation. We consider t
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Giant Gilbert damping anisotropy is identified as a signature of strong Rashba spin-orbit coupling in a two-dimensional antiferromagnet on a honeycomb lattice. The phenomenon originates in spin-orbit induced splitting of conduction electron subbands that strongly suppresses certain spin-flip processes. As a result, the spin-orbit interaction is shown to support an undamped non-equilibrium dynamical mode that corresponds to an ultrafast in-plane Neel vector precession and a constant perpendicular-to-the-plane magnetization. The phenomenon is illustrated on the basis of a two dimensional $s$-$d$ like model. Spin-orbit torques and conductivity are also computed microscopically for this model. Unlike Gilbert damping these quantities are shown to reveal only a weak anisotropy that is limited to the semiconductor regime corresponding to the Fermi energy staying in a close vicinity of antiferromagnetic gap.
The current family of experimentally realized two-dimensional magnetic materials consist of 3$d$ transition metals with very weak spin-orbit coupling. In contrast, we report a new platform in a chemically bonded and layered 4$d$ oxide, with strong electron correlations and competing spin-orbit coupling. We synthesize ultra-thin sheets of SrRu$_2$O$_6$ using scalable liquid exfoliation. These exfoliated sheets are characterized by complementary experimental and theoretical techniques. The thickness of the nano-sheets varies between three to five monolayers, and within the first-principles calculations, we show that antiferromagnetism survives in these ultra-thin layers. Experimental data suggest that exfoliation occurs from the planes perpendicular to the $c$-axis as the intervening hexagonal Sr-lattice separates the two-dimensional magnetic honeycomb Ru-layers. The high-resolution transmission electron microscope images indicate that the average inter-atomic spacing between the Ru-layers is slightly reduced, which agrees with the present calculations. The signatures of rotational stacking of the nanosheets are also observed. Such new two-dimensional platform offers enormous possibilities to explore emergent properties that appear due to the interplay between magnetism, strong correlations and spin-orbit coupling. Moreover, these effects can be further tuned as a function of layer thickness.
The quantum mechanical screening of a spin via conduction electrons depends sensitively on the environment seen by the magnetic impurity. A high degree of responsiveness can be obtained with metal complexes, as the embedding of a metal ion into an organic molecule prevents intercalation or alloying and allows for a good control by an appropriate choice of the ligands. There are therefore hopes to reach an on demand control of the spin state of single molecules adsorbed on substrates. Hitherto one route was to rely on switchable molecules with intrinsic bistabilities triggered by external stimuli, such as temperature or light, or on the controlled dosing of chemicals to form reversible bonds. However, these methods constrain the functionality to switchable molecules or depend on access to atoms or molecules. Here, we present a way to induce bistability also in a planar molecule by making use of the environment. We found that the particular habitat offered by an antiphase boundary of the Rashba system BiAg$_2$ stabilizes a second structure for manganese phthalocyanine molecules, in which the central Mn ion moves out of the molecular plane. This corresponds to the formation of a large magnetic moment and a concomitant change of the ground state with respect to the conventional adsorption site. The reversible spin switch found here shows how we can not only rearrange electronic levels or lift orbital degeneracies via the substrate, but even sway the effects of many-body interactions in single molecules by acting on their surrounding.
Current induced spin-orbit torques have been studied in ferromagnetic nanowires made of 20 nm thick Co/Pd multilayers with perpendicular magnetic anisotropy. Using Hall voltage and lock-in measurements, it is found that upon injection of an electric current both in-plane (Slonczewski-like) and perpendicular (field-like) torques build up in the nanowire. The torque efficiencies are found to be as large as 1.17 kOe and 5 kOe at 108 A/cm2 for the in-plane and perpendicular components, respectively, which is surprisingly comparable to previous studies in ultrathin (~ 1 nm) magnetic bilayers. We show that this result cannot be explained solely by spin Hall effect induced torque at the outer interfaces, indicating a probable contribution of the bulk of the Co/Pd multilayer.
We report the enhancement of spin-orbit torques in MnAl/Ta films with improving chemical ordering through annealing. The switching current density is increased due to enhanced saturation magnetization MS and effective anisotropy field HK after annealing. Both damplinglike effective field HD and fieldlike effective field HF have been increased in the temperature range of 50 to 300 K. HD varies inversely with MS in both of the films, while the HF becomes liner dependent on 1/MS in the annealed film. We infer that the improved chemical ordering has enhanced the interfacial spin transparency and the transmitting of the spin current in MnAl layer.
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