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Transport theory for femtosecond laser-induced spin-transfer torques

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 Added by Pavel Balaz
 Publication date 2017
  fields Physics
and research's language is English




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Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear magnetizations. To this end, we introduce an extended model of superdiffusive spin transport that enables to treat noncollinear magnetic configurations, and apply it to the perpendicular spin valve geometry. We show how spin-transfer torques arise due to this mechanism and calculate their action on the magnetization present, as well as how the latter depends on the thicknesses of the layers and other transport parameters. We demonstrate that there exists a certain optimum thickness of the out-of-plane magnetized spin-current polarizer such that the torque acting on the second magnetic layer is maximal. Moreover, we study the magnetization dynamics excited by the superdiffusive spin-transfer torque due to the flow of hot electrons employing the Landau-Lifshitz-Gilbert equation. Thereby we show that a femtosecond laser pulse applied to one magnetic layer can excite small-angle precessions of the magnetization in the second magnetic layer. We compare our calculations with recent experimental results.



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Manipulation of magnetic domain walls via a helicity-independent laser pulse has recently been experimentally demonstrated and various physical mechanisms leading to domain wall dynamics have been discussed. Spin-dependent superdiffusive transport of hot electrons has been identified as one of the possible ways how to affect a magnetic domain wall. Here, we develop a model based on superdiffusive spin-dependent transport to study the laser-induced transport of hot electrons through a smooth magnetic domain wall. We show that the spin transfer between neighboring domains can enhance ultrafast demagnetization in the domain wall. More importantly, our calculations reveal that when the laser pulse is properly focused on to the vicinity of the domain wall, it can excite sufficiently strong spin currents to generate a spin-transfer torque that can rapidly move the magnetic domain wall by several nanometers in several hundreds of femtoseconds, leading to a huge nonequilibrium domain wall velocity.
Current-induced torques on ferromagnetic nanoparticles and on domain walls in ferromagnetic nanowires are normally understood in terms of transfer of conserved spin angular momentum between spin-polarized currents and the magnetic condensate. In a series of recent articles we have discussed a microscopic picture of current-induced torques in which they are viewed as following from exchange fields produced by the misaligned spins of current carrying quasiparticles. This picture has the advantage that it can be applied to systems in which spin is not approximately conserved. More importantly, this point of view makes it clear that current-induced torques can also act on the order parameter of an antiferromagnetic metal, even though this quantity is not related to total spin. In this informal and intentionally provocative review we explain this picture and discuss its application to antiferromagnets.
We investigate laser-induced torques in magnetically non-collinear ferromagnets with a spin-spiral magnetic structure using textit{ab-initio} calculations. Since spin-spirals may be used to approximate the magnetization gradients locally in domain walls and skyrmions, our method may be used to obtain the laser-induced torques in such objects from a multiscale approach. Employing the generalized Bloch-theorem we obtain the electronic structure computationally efficiently. We employ our method to assess the laser-induced torques in bcc Fe, hcp Co, and L$_{1}0$ FePt when a spin-spiral magnetic structure is imposed. We find that the laser-induced torques in these magnetically noncollinear systems may be orders of magnitude larger than those in the corresponding magnetically collinear systems and that they exist both for linearly and circularly polarized light. This result suggests that laser-induced torques driven by noncollinear magnetic order or by magnetic fluctuations may contribute significantly to processes in ultrafast magnetism.
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