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Register a new userFirst-principles quantum transport modeling of spin-transfer and spin-orbit torques in magnetic multilayers
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We review a unified approach for computing: (i) spin-transfer torque in magnetic trilayers like spin-valves and magnetic tunnel junction, where injected charge current flows perpendicularly to interfaces; and (ii) spin-orbit torque in magnetic bilayers of the type ferromagnet/spin-orbit-coupled-material, where injected charge current flows parallel to the interface. Our approach requires to construct the torque operator for a given Hamiltonian of the device and the steady-state nonequilibrium density matrix, where the latter is expressed in terms of the nonequilibrium Greens functions and split into three contributions. Tracing these contributions with the torque operator automatically yields field-like and damping-like components of spin-transfer torque or spin-orbit torque vector, which is particularly advantageous for spin-orbit torque where the direction of these components depends on the unknown-in-advance orientation of the current-driven nonequilibrium spin density in the presence of spin-orbit coupling. We provide illustrative examples by computing spin-transfer torque in a one-dimensional toy model of a magnetic tunnel junction and realistic Co/Cu/Co spin-valve, both of which are described by first-principles Hamiltonians obtained from noncollinear density functional theory calculations; as well as spin-orbit torque in a ferromagnetic layer described by a tight-binding Hamiltonian which includes spin-orbit proximity effect within ferromagnetic monolayers assumed to be generated by the adjacent monolayer transition metal dichalcogenide.
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Spin-orbit interaction (SOI) couples charge and spin transport, enabling electrical control of magnetization. A quintessential example of SOI-induced transport is the anomalous Hall effect (AHE), first observed in 1880, in which an electric current perpendicular to the magnetization in a magnetic film generates charge accumulation on the surfaces. Here we report the observation of a counterpart of the AHE that we term the anomalous spin-orbit torque (ASOT), wherein an electric current parallel to the magnetization generates opposite spin-orbit torques on the surfaces of the magnetic film. We interpret the ASOT as due to a spin-Hall-like current generated with an efficiency of 0.053+/-0.003 in Ni80Fe20, comparable to the spin Hall angle of Pt. Similar effects are also observed in other common ferromagnetic metals, including Co, Ni, and Fe. First principles calculations corroborate the order of magnitude of the measured values. This work suggests that a strong spin current with spin polarization transverse to magnetization can exist in a ferromagnet, despite spin dephasing. It challenges the current understanding of spin-orbit torque in magnetic/nonmagnetic bilayers, in which the charge-spin conversion in the magnetic layer has been largely neglected.
Electron transport in magnetic orders and the magnetic orders dynamics have a mutual dependence, which provides the key mechanisms in spin-dependent phenomena. Recently, antiferromagnetic orders are focused on as the magnetic order, where current-induced spin-transfer torques, a typical effect of electron transport on the magnetic order, have been debatable mainly because of the lack of an analytic derivation based on quantum field theory. Here, we construct the microscopic theory of spin-transfer torques on the slowly-varying staggered magnetization in antiferromagnets with weak canting. In our theory, the electron is captured by bonding/antibonding states, each of which is the eigenstate of the system, doubly degenerates, and spatially spreads to sublattices because of electron hopping. The spin of the eigenstates depends on the momentum in general, and a nontrivial spin-momentum locking arises for the case with no site inversion symmetry, without considering any spin-orbit couplings. The spin current of the eigenstates includes an anomalous component proportional to a kind of gauge field defined by derivatives in momentum space and induces the adiabatic spin-transfer torques on the magnetization. Unexpectedly, we find that one of the nonadiabatic torques has the same form as the adiabatic spin-transfer torque, while the obtained forms for the adiabatic and nonadiabatic spin-transfer torques agree with the phenomenological derivation based on the symmetry consideration. This finding suggests that the conventional explanation for the spin-transfer torques in antiferromagnets should be changed. Our microscopic theory provides a fundamental understanding of spin-related physics in antiferromagnets.
We measure spin-orbit torques (SOTs) in a unique model system of all-epitaxial ferrite/Pt bilayers to gain insights into charge-spin interconversion in Pt. With negligible electronic conduction in the insulating ferrite, the crystalline Pt film acts as the sole source of charge-to-spin conversion. A small field-like SOT independent of Pt thickness suggests a weak Rashba-Edelstein effect at the ferrite/Pt interface. By contrast, we observe a sizable damping-like SOT that depends on the Pt thickness, from which we deduce the dominance of an extrinsic spin-Hall effect (skew scattering) and Dyakonov-Perel spin relaxation in the crystalline Pt film. Furthermore, our results point to a large internal spin-Hall ratio of $approx$0.8 in epitaxial Pt. Our experimental work takes an essential step towards understanding the mechanisms of charge-spin interconversion and SOTs in Pt-based heterostructures, which are crucial for power-efficient spintronic devices.
We study the optically induced torques in thin film ferromagnetic layers under excitation by circularly polarized light. We study cases both with and without Rashba spin-orbit coupling using a 4-band model. In the absence of Rashba spin-orbit coupling, we derive an analytic expression for the optical torques, revealing the conditions under which the torque is mostly derived from optical spin transfer torque (i.e. when the torque is along the direction of optical angular momentum), versus when the torque is derived from the inverse Faraday effect (i.e. when the torque is perpendicular to the optical angular momentum). We find the optical spin transfer torque dominates provided that the excitation energy is far away from band edge transitions, and the magnetic exchange splitting is much greater than the lifetime broadening. For the case with large Rashba spin-orbit coupling and out-of-plane magnetization, we find the torque is generally perpendicular to the photon angular momentum and is ascribed to an optical Edelstein effect.
We reported a systematic study of spin-orbit torque biased magnetic sensors based on NiFe/Pt bilayers through both macro-spin modeling and experiments. The simulation results show that it is possible to achieve a linear sensor with a dynamic range of 0.1 - 10 Oe, power consumption of 1uW - 1 mW, and sensitivity of 0.1-0.5 Ohm/Oe. These characteristics can be controlled by varying the sensor dimension and current density in the Pt layer. The latter is in the range of 1 x 10^5 - 10^7 A/cm^2. Experimental results of fabricated sensors with selected sizes agree well with the simulation results. For a Wheatstone bridge sensor comprising of four sensing elements, a sensitivity up to 0.548 Ohm/Oe, linearity error below 6%, and detectivity of about 2.8 nT/Sqrt(Hz) were obtained. The simple structure and ultrathin thickness greatly facilitate the integration of these sensors for on-chip applications. As a proof-of-concept experiment, we demonstrate its application in detection of current flowing in an on-chip Cu wire.
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