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Register a new userStudy of fusion-fission in inverse kinematics with a fragment separator
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The systematic study of fission fragment yields under different initial conditions provides a valuable experimental benchmark for fission models that aim to understand this complex decay channel and to predict reaction product yields. Inverse kinematics coupled to the use of a high-resolution spectrometer is shown to be a powerful tool to identify and measure the inclusive isotopic yields of fission fragments. In-flight fusion fission was used to produce secondary beams of neutron-rich isotopes in the collision of a 238U beam at 24 MeV/u with 9Be and 12C targets at GANIL using the LISE3 fragment-separator. Unique A,Z,q identification of fission products was attained with the dE-TKE-Brho-ToF measurement technique. Mass, and atomic number distributions are reported for the two reactions that show the importance of different reaction mechanisms for these two targets.
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During the fission process, the nucleus deforms and elongates up to the two fragments inception and their final separation at scission deformation. The evolution of the nucleus energy with deformation is determined by the macroscopic properties of the nucleus, and is also strongly influenced by the single-particle structure of the nucleus. The fission fragment distribution is a direct consequence of the deformation path the nucleus has encountered, and therefore is the most genuine experimental observation of the potential energy landscape of the deforming nucleus. Very asymmetric fusion-fission reactions at energy close to the Coulomb barrier, produce well-defined conditions of the compound nucleus formation, where processes such as quasi-fission, pre-equilibrium emission and incomplete fusion are negligible. In the same time, the excitation energy is sufficient to reduce significantly structural effects, and mostly the macroscopic part of the potential is responsible for the formation of the fission fragments. We use inverse kinematics combined with spectrometers to select and identify the fission fragments produced in $^{238}$U+$^{12}$C at a bombarding energy close to and well-above the Coulomb barrier. For the first time, the isotopic yields are measured over the complete atomic-number distribution, between Z=30 and Z=63. The experimental set-up also allows to identify transfer-induced reactions, which lead to low-energy fission where the nuclear shell structure shows a strong influence on the fission-fragment distributions. The resulting set of data gives the possibility to observe the fission fragment properties over a wide range of excitation energy, and they reveal the vanishing of the shell effects in the potential energy of the fissioning nucleus, as well as the influence of fission dynamics.
A novel method to access the complete identification in atomic number Z and mass A of fragments produced in low-energy fission of actinides is presented. This method, based on the use of multi- nucleon transfer and fusion reactions in inverse kinematics, is applied in this work to reactions between a 238U beam and a 12C target to produce and induce fission of moderately excited actinides. The fission fragments are detected and fully identified with the VAMOS spectrometer of GANIL, allowing the measurement of fragment yields of several hundreds of isotopes in a range between A ~ 80 and ~ 160, and from Z ~ 30 to ~ 64. For the first time, complete isotopic yield distributions of fragments from well-defined fissioning systems are available. Together with the precise measurement of the fragment emission angles and velocities, this technique gives further insight into the nuclear-fission process.
Inelastic and multi-nucleon transfer reactions between a $^{238}$U beam, accelerated at 6.14 MeV/u, and a $^{12}$C target were used for the production of neutron-rich, fissioning systems from U to Cm. A Si telescope, devoted to the detection of the target-like nuclei, provided a characterization of the fissioning systems in atomic and mass numbers, as well as in excitation energy. Cross-sections, angular and excitation-energy distributions were measured for the inelastic and transfer channels. Possible excitations of the target-like nuclei were experimentally investigated for the first time, by means of g -ray measurements. The decays from the first excited states of $^{12}$C, $^{11}$B and $^{10}$Be were observed with probabilities of 0.12 - 0.14, while no evidence for the population of higher-lying states was found. Moreover, the fission probabilities of $^{238}$U, $^{239}$Np and $^{240,241,242}$Pu and $^{244}$Cm were determined as a function of the excitation energy.
Fission fragment angular distributions can provide an important constraint on fission theory, improving predictive fission codes, and are a prerequisite for a precise ratio cross section measurement. Available anisotropy data is sparse, especially at neutron energies above 5 MeV. For the first time, a three-dimensional tracking detector is employed to study fragment emission angles and provide a direct measurement of angular anisotropy. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has deployed the fission time projection chamber (fissionTPC) to measure nuclear data with unprecedented precision. The fission fragment anisotropy of $^{235}$U has been measured over a wide range of incident neutron energies from 180 keV to 200 MeV; a careful study of the systematic uncertainties complement the data.
The fission fragment mass distributions have been measured in the reactions 16O + 184W and 19F+ 181Ta populating the same compound nucleus 200Pb? at similar excitation energies. It is found that the widths of the mass distribution increases monotonically with excitation energy, indicating the absence of quasi-fission for both reactions. This is contrary to two recent claims of the presence of quasi-fission in the above mentioned reactions.
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