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Register a new userIsotopic fission fragment distributions as a deep probe to fusion-fission dynamics
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During the fission process, the nucleus deforms and elongates up to the two fragments inception and their final separation at scission deformation. The evolution of the nucleus energy with deformation is determined by the macroscopic properties of the nucleus, and is also strongly influenced by the single-particle structure of the nucleus. The fission fragment distribution is a direct consequence of the deformation path the nucleus has encountered, and therefore is the most genuine experimental observation of the potential energy landscape of the deforming nucleus. Very asymmetric fusion-fission reactions at energy close to the Coulomb barrier, produce well-defined conditions of the compound nucleus formation, where processes such as quasi-fission, pre-equilibrium emission and incomplete fusion are negligible. In the same time, the excitation energy is sufficient to reduce significantly structural effects, and mostly the macroscopic part of the potential is responsible for the formation of the fission fragments. We use inverse kinematics combined with spectrometers to select and identify the fission fragments produced in $^{238}$U+$^{12}$C at a bombarding energy close to and well-above the Coulomb barrier. For the first time, the isotopic yields are measured over the complete atomic-number distribution, between Z=30 and Z=63. The experimental set-up also allows to identify transfer-induced reactions, which lead to low-energy fission where the nuclear shell structure shows a strong influence on the fission-fragment distributions. The resulting set of data gives the possibility to observe the fission fragment properties over a wide range of excitation energy, and they reveal the vanishing of the shell effects in the potential energy of the fissioning nucleus, as well as the influence of fission dynamics.
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The fission fragment mass distributions have been measured in the reactions 16O + 184W and 19F+ 181Ta populating the same compound nucleus 200Pb? at similar excitation energies. It is found that the widths of the mass distribution increases monotonically with excitation energy, indicating the absence of quasi-fission for both reactions. This is contrary to two recent claims of the presence of quasi-fission in the above mentioned reactions.
A direct and complete measurement of isotopic fission-fragment yields of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced with an average excitation energy of 8.3 MeV in one-neutron transfer reactions between a $^{238}$U beam and a $^{9}$Be target at Coulomb barrier energies. The fission fragments were detected and isotopically identified using the VAMOS++ spectrometer at the GANIL facility. This measurement allows to directly evaluate the fission models at excitation energies of fast neutrons, relevant for next-generation nuclear reactors. The present data, in agreement with model calculations, do not support the recently reported anomaly in the fission-fragment yields of $^{239}$U and confirm the persistence of spherical shell effects in the Sn region at excitation energies exceeding the fission barrier by few MeV.
The systematic study of fission fragment yields under different initial conditions provides a valuable experimental benchmark for fission models that aim to understand this complex decay channel and to predict reaction product yields. Inverse kinematics coupled to the use of a high-resolution spectrometer is shown to be a powerful tool to identify and measure the inclusive isotopic yields of fission fragments. In-flight fusion fission was used to produce secondary beams of neutron-rich isotopes in the collision of a 238U beam at 24 MeV/u with 9Be and 12C targets at GANIL using the LISE3 fragment-separator. Unique A,Z,q identification of fission products was attained with the dE-TKE-Brho-ToF measurement technique. Mass, and atomic number distributions are reported for the two reactions that show the importance of different reaction mechanisms for these two targets.
The dynamics of the fission process is expected to affect the evaporation residue cross section because of the fission hindrance due to the nuclear viscosity. Systems of intermediate fissility constitute a suitable environment for testing such hypothesis, since they are characterized by evaporation residue cross sections comparable or larger than the fission ones. Observables related to emitted charged particle, due to their relatively high emission probability, can be used to put stringent constraints on models describing the excited nucleus decay and to recognize the effects of fission dynamics. In this work model simulations are compared with the experimental data collected via the ^{32}S + ^{100}Mo reaction at E_{lab}= 200 MeV. By comparing an extended set of evaporation channel observables the limits of the statistical model and the large improvement coming by using a dynamical model are evidenced. The importance of using a large angular covering apparatus to extract the observable is stressed. The opportunity to measure more sensitive observables by a new detection device in operation at LNL are also discussed.
A novel method to access the complete identification in atomic number Z and mass A of fragments produced in low-energy fission of actinides is presented. This method, based on the use of multi- nucleon transfer and fusion reactions in inverse kinematics, is applied in this work to reactions between a 238U beam and a 12C target to produce and induce fission of moderately excited actinides. The fission fragments are detected and fully identified with the VAMOS spectrometer of GANIL, allowing the measurement of fragment yields of several hundreds of isotopes in a range between A ~ 80 and ~ 160, and from Z ~ 30 to ~ 64. For the first time, complete isotopic yield distributions of fragments from well-defined fissioning systems are available. Together with the precise measurement of the fragment emission angles and velocities, this technique gives further insight into the nuclear-fission process.
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