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From confined spinons to emergent fermions: Observation of elementary magnetic excitations in a transverse-field Ising chain

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 Added by Zhe Wang
 Publication date 2015
  fields Physics
and research's language is English




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We report on spectroscopy study of elementary magnetic excitations in an Ising-like antiferromagnetic chain compound SrCo$_2$V$_2$O$_8$ as a function of temperature and applied transverse magnetic field up to 25 T. An optical as well as an acoustic branch of confined spinons, the elementary excitations at zero field, are identified in the antiferromagnetic phase below the N{e}el temperature of 5 K and described by a one-dimensional Schr{o}dinger equation. The confinement can be suppressed by an applied transverse field and a quantum disordered phase is induced at 7 T. In this disordered paramagnetic phase, we observe three emergent fermionic excitations with different transverse-field dependencies. The nature of these modes is clarified by studying spin dynamic structure factor of a 1D transverse-field Heisenberg-Ising (XXZ) model using the method of infinite time evolving block decimation. Our work reveals emergent quantum phenomena and provides a concrete system for testifying theoretical predications of one-dimension quantum spin models.



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We study the dynamics of the quasi-one-dimensional Ising-Heisenberg antiferromagnet BaCo2V2O8 under a transverse magnetic field. Combining inelastic neutron scattering experiments and theoretical analyses by field theories and numerical simulations, we mainly elucidate the structure of the spin excitation spectrum in the high field phase, appearing above the quantum phase transition point mu0Hc ~ 10 T. We find that it is characterized by collective solitonic excitations superimposed on a continuum. These solitons are strongly bound in pairs due to the effective staggered field induced by the nondiagonal g tensor of the compound, and are topologically different from the fractionalized spinons in the weak field region. The dynamical susceptibility numerically calculated with the infinite time-evolving block decimation method shows an excellent agreement with the measured spectra, which enables us to identify the dispersion branches with elementary excitations. The lowest energy dispersion has an incommensurate nature and has a local minimum at an irrational wave number due to the applied transverse field.
We develop a technique to directly study spinons (emergent spin S = 1/2 particles) in quantum spin models in any number of dimensions. The size of a spinon wave packet and of a bound pair (a triplon) are defined in terms of wave-function overlaps that can be evaluated by quantum Monte Carlo simulations. We show that the same information is contained in the spin-spin correlation function as well. We illustrate the method in one dimension. We confirm that spinons are well defined particles (have exponentially localized wave packet) in a valence-bond-solid state, are marginally defined (with power-law shaped wave packet) in the standard Heisenberg critical state, and are not well defined in an ordered Neel state (achieved in one dimension using long-range interactions).
We report on magnetization, sound velocity, and magnetocaloric-effect measurements of the Ising-like spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8$ as a function of temperature down to 1.3 K and applied transverse magnetic field up to 60 T. While across the N{e}el temperature of $T_Nsim5$ K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity $v(B)$ and a clear minimum of temperature $T(B)$ at $B^{c,3D}_perp=21.4$ T, indicating the suppression of the antiferromagnetic order. At higher fields, the $T(B)$ curve shows a broad minimum at $B^c_perp = 40$ T, accompanied by a broad minimum in the sound velocity and a saturation-like magnetization. These features signal a quantum phase transition which is further characterized by the divergent behavior of the Gr{u}neisen parameter $Gamma_B propto (B-B^{c}_perp)^{-1}$. By contrast, around the critical field, the Gr{u}neisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.
141 - Zhe Wang , M. Schmidt , A. Loidl 2019
We report a high-resolution terahertz spectroscopic study of quantum spin dynamics in the antiferromagnetic Heisenberg-Ising spin-chain compound BaCo$_2$V$_2$O$_8$ as a function of temperature and longitudinal magnetic field. Confined spinon excitations are observed in an antiferromagnetic phase below $T_Nsimeq 5.5$ K. In a field-induced gapless phase above $B_c=3.8$ T, we identify many-body string excitations as well as low-energy fractional psinon/antipsinon excitations by comparing to Bethe-Ansatz calculations. In the vicinity of $B_c$, the high-energy string excitations are found to be dynamically dominant over the fractional excitations.
The field-induced transition in one-dimensional S=1 Heisenberg antiferromagnet with single-ion anisotropy in the presence of a transverse magnetic field is obtained on the basis of the Schwinger boson mean-field theory. The behaviors of the specific heat and susceptibility as functions of temperature as well as the applied transverse field are explored, which are found to be different from the results obtained under a longitudinal field. The anomalies of the specific heat at low temperatures, which might be an indicative of a field-induced transition from a Luttinger liquid phase to an ordered phase, are explicitly uncovered under the transverse field. A schematic phase diagram is proposed. The theoretical results are compared with experimental observations.
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