No Arabic abstract
We study the dynamics of the quasi-one-dimensional Ising-Heisenberg antiferromagnet BaCo2V2O8 under a transverse magnetic field. Combining inelastic neutron scattering experiments and theoretical analyses by field theories and numerical simulations, we mainly elucidate the structure of the spin excitation spectrum in the high field phase, appearing above the quantum phase transition point mu0Hc ~ 10 T. We find that it is characterized by collective solitonic excitations superimposed on a continuum. These solitons are strongly bound in pairs due to the effective staggered field induced by the nondiagonal g tensor of the compound, and are topologically different from the fractionalized spinons in the weak field region. The dynamical susceptibility numerically calculated with the infinite time-evolving block decimation method shows an excellent agreement with the measured spectra, which enables us to identify the dispersion branches with elementary excitations. The lowest energy dispersion has an incommensurate nature and has a local minimum at an irrational wave number due to the applied transverse field.
We report on spectroscopy study of elementary magnetic excitations in an Ising-like antiferromagnetic chain compound SrCo$_2$V$_2$O$_8$ as a function of temperature and applied transverse magnetic field up to 25 T. An optical as well as an acoustic branch of confined spinons, the elementary excitations at zero field, are identified in the antiferromagnetic phase below the N{e}el temperature of 5 K and described by a one-dimensional Schr{o}dinger equation. The confinement can be suppressed by an applied transverse field and a quantum disordered phase is induced at 7 T. In this disordered paramagnetic phase, we observe three emergent fermionic excitations with different transverse-field dependencies. The nature of these modes is clarified by studying spin dynamic structure factor of a 1D transverse-field Heisenberg-Ising (XXZ) model using the method of infinite time evolving block decimation. Our work reveals emergent quantum phenomena and provides a concrete system for testifying theoretical predications of one-dimension quantum spin models.
The quantum criticality of an Ising-like screw chain antiferromagnet SrCo$_2$V$_2$O$_8$, with a transverse magnetic field applied along the crystalline $a$-axis, is investigated by ultra-low temperature NMR measurements. The N{e}el temperature is rapidly and continuously suppressed by the field, giving rise to a quantum critical point (QCP) at $H_{C{_1}}$$approx$~7.0~T. Surprisingly, a second QCP at $H_{C{_2}}approx$~7.7~T featured with gapless excitations is resolved from both the double-peak structure of the field dependent spin-lattice relaxation rate $1/^{51}T_1$ at low temperatures and the weakly temperature-dependent $1/^{51}T_1$ at this field. Our data, combined with numerical calculations, suggest that the induced effective staggered transverse field significantly lowers the critical fields, and leads to an exposed QCP at $H_{C{_2}}$, which belongs to the one-dimensional transverse-field Ising universality.
We report on magnetization, sound velocity, and magnetocaloric-effect measurements of the Ising-like spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8$ as a function of temperature down to 1.3 K and applied transverse magnetic field up to 60 T. While across the N{e}el temperature of $T_Nsim5$ K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity $v(B)$ and a clear minimum of temperature $T(B)$ at $B^{c,3D}_perp=21.4$ T, indicating the suppression of the antiferromagnetic order. At higher fields, the $T(B)$ curve shows a broad minimum at $B^c_perp = 40$ T, accompanied by a broad minimum in the sound velocity and a saturation-like magnetization. These features signal a quantum phase transition which is further characterized by the divergent behavior of the Gr{u}neisen parameter $Gamma_B propto (B-B^{c}_perp)^{-1}$. By contrast, around the critical field, the Gr{u}neisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.
BaCo2V2O8 is a nice example of a quasi-one-dimensional quantum spin system that can be described in terms of Tomonaga-Luttinger liquid physics. This is explored in the present study where the magnetic field-temperature phase diagram is thoroughly established up to 12 T using single-crystal neutron diffraction. The transition from the Neel phase to the incommensurate longitudinal spin density wave (LSDW) phase through a first-order transition, as well as the critical exponents associated with the paramagnetic to ordered phase transitions, and the magnetic order both in the Neel and in the LSDW phase are determined, thus providing a stringent test for the theory.
We report a combination of physical property and neutron scattering measurements for polycrystalline samples of the one-dimensional spin chain compound CoV2O6. Heat capacity measurements show that an effective S = 1/2 state is found at low temperatures and that magnetic fluctuations persist up to 6.Tn. Above Tn = 6.3 K, measurements of the magnetic susceptibility as a function of T and H show that the nearest neighbour exchange is ferromagnetic. In the ordered state, we have discovered a crossover from a metamagnet with strong fluctuations between 5 K and Tn to a state with a 1/3 magnetisation plateau at 2 < T < 5 K. We use neutron powder diffraction measurements to show that the AFM state has incommensurate long range order and inelastic time of flight neutron scattering to examine the magnetic fluctuations as a function of temperature. Above Tn, we find two broad bands between 3.5 and 5 meV and thermally activated low energy features which correspond to transitions within these bands. These features show that the excitations are deconfined solitons rather than the static spin reversals predicted for a uniform FM Ising spin chain. Below Tn, we find a ladder of states due to the confining effect of the internal field. A region of weak confinement below Tn, but above 5 K, is identified which may correspond to a crossover between 2D and 3D magnetic ordering.