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Register a new userIndirect quantum sensors: Improving the sensitivity in characterizing very weakly coupled spins
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Added by
Johannes N. Greiner
Publication date
2015
fields
Physics
and research's language is
English
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We propose a scheme to increase the sensitivity and thus the detection volume of nanoscale single molecule magnetic resonance imaging. The proposal aims to surpass the T1 limited detection of the sensor by taking advantage of a long-lived ancilla nuclear spin to which the sensor is coupled. We show how this nuclear spin takes over the role of the sensor spin, keeping the characteristic time-scales of detection on the same order but with a longer life-time allowing it to detect a larger volume of the sample which is not possible by the sensor alone.
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We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled relaxation and achieve a polarity-tunable, fast nuclear polarization of degree higher than 85% at room temperature for remote 13C nuclear spins exhibiting hyperfine interaction strength with NV centers of the order of 600 kHz. We show with the aid of numerical simulation that the anisotropic hyperfine tensor components naturally provide a route to control spin mixing parameter so that highly efficient nuclear polarization is enabled through careful tuning of nuclear quantization axis by external magnetic field. We further discuss spin dynamics and wide applicability of this method to various target 13C nuclear spins around the NV center electron spin. The proposed control method demonstrates an efficient and versatile route to realize, for example, high-fidelity spin register initialization and quantum metrology using nuclear spin resources in solids.
In the field of cavity optomechanics, proposals for quantum nondemolition (QND) measurements of phonon number provide a promising avenue by which one can study the quantum nature of nanoscale mechanical resonators. Here, we investigate these QND measurements for an optomechanical system whereby quadratic coupling arises due to shared symmetries between a single optical resonance and a mechanical mode. We establish a relaxed limit on the amount of linear coupling that can exist in this type of system while still allowing for a QND measurement of Fock states. This new condition enables optomechanical QND measurements, which can be used to probe the decoherence of mesoscopic mechanical Fock states, providing an experimental testbed for quantum collapse theories.
The extraordinary sensitivity of plasmonic sensors is well known in the optics and photonics community. These sensors exploit simultaneously the enhancement and the localization of electromagnetic fields close to the interface between a metal and a dielectric. This enables, for example, the design of integrated biochemical sensors at scales far below the diffraction limit. Despite their practical realization and successful commercialization, the sensitivity and associated precision of plasmonic sensors are starting to reach their fundamental classical limit given by quantum fluctuations of light -- known as the shot-noise limit. To improve the sensing performance of these sensors beyond the classical limit, quantum resources are increasingly being employed. This area of research has become known as `quantum plasmonic sensing and it has experienced substantial activity in recent years for applications in chemical and biological sensing. This review aims to cover both plasmonic and quantum techniques for sensing, and shows how they have been merged to enhance the performance of plasmonic sensors beyond traditional methods. We discuss the general framework developed for quantum plasmonic sensing in recent years, covering the basic theory behind the advancements made, and describe the important works that made these advancements. We also describe several key works in detail, highlighting their motivation, the working principles behind them, and their future impact. The intention of the review is to set a foundation for a burgeoning field of research that is currently being explored out of intellectual curiosity and for a wide range of practical applications in biochemistry, medicine, and pharmaceutical research.
Single epitaxially-grown semiconductor quantum dots have great potential as single photon sources for photonic quantum technologies, though in practice devices often exhibit non-ideal behavior. Here, we demonstrate that amplitude modulation can improve the performance of quantum-dot-based sources. Starting with a bright source consisting of a single quantum dot in a fiber-coupled microdisk cavity, we use synchronized amplitude modulation to temporally filter the emitted light. We observe that the single photon purity, temporal overlap between successive emission events, and indistinguishability can be greatly improved with this technique. As this method can be applied to any triggered single photon source, independent of geometry and after device fabrication, it is a flexible approach to improve the performance of solid-state systems, which often suffer from excess dephasing and multi-photon background emission.
Cavities embedded in photonic crystal waveguides offer a promising route towards large scale integration of coupled resonators for quantum electrodynamics applications. In this letter, we demonstrate a strongly coupled system formed by a single quantum dot and such a photonic crystal cavity. The resonance originating from the cavity is clearly identified from the photoluminescence mapping of the out-of-plane scattered signal along the photonic crystal waveguide. The quantum dot exciton is tuned towards the cavity mode by temperature control. A vacuum Rabi splitting of ~ 140 mueV is observed at resonance.
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