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Register a new userDecoherence-assisted spectroscopy of a single Mg$^+$ ion
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We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly at rest are recorded efficiently with high signal-to-noise ratios. Spectra display symmetric line shapes without stray-light background from spectroscopy probes. We employ this method on a $^{25}$Mg$^+$ ion to measure one, two, and three-photon transition frequencies from the 3S ground state to the 3P, 3D, and 4P excited states, respectively. Our results are relevant for astrophysics and searches for drifts of fundamental constants. Furthermore, the method can be extended to other transitions, isotopes, and species. The currently achieved fractional frequency uncertainty of $5 times 10^{-9}$ is not limited by the method.
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We use a co-trapped ion ($^{88}mathrm{Sr}^{+}$) to sympathetically cool and measure the quantum state populations of a memory-qubit ion of a different atomic species ($^{40}mathrm{Ca}^{+}$) in a cryogenic, surface-electrode ion trap. Due in part to the low motional heating rate demonstrated here, the state populations of the memory ion can be transferred to the auxiliary ion by using the shared motion as a quantum state bus and measured with an average accuracy of 96(1)%. This scheme can be used in quantum information processors to reduce photon-scattering-induced error in unmeasured memory qubits.
We compute the Rydberg spectrum of a single Ca$^+$ ion in a Paul trap by incorporating various internal and external coupling terms of the ion to the trap in the Hamiltonian. The coupling terms include spin-orbit coupling in Ca$^+$, charge (electron and ionic core) coupling to the radio frequency and static fields, ion-electron coupling in the Paul trap, and ion center-of-mass coupling. The electronic Rydberg states are precisely described by a one-electron model potential for e$^-$+Ca$^{2+}$, and accurate eigenenergies, quantum defect parameters, and static and tensor polarizabilities for a number of excited Rydberg states are obtained. The time-periodic rf Hamiltonian is expanded in the Floquet basis, and the trapping-field-broadened Rydberg lines are compared with recent observations of Ca$^+(23P)$ and Ca$^+(52F)$ Rydberg lines.
We provide a comprehensive theoretical framework for describing the dynamics of a single trapped ion interacting with a neutral buffer gas, thus extending our previous studies on buffer-gas cooling of ions beyond the critical mass ratio [B. Holtkemeier et al., Phys. Rev. Lett. 116, 233003 (2016)]. By transforming the collisional processes into a frame, where the ions micromotion is assigned to the buffer gas atoms, our model allows one to investigate the influence of non-homogeneous buffer gas configurations as well as higher multipole orders of the radio-frequency trap in great detail. Depending on the neutral-to-ion mass ratio, three regimes of sympathetic cooling are identified which are characterized by the form of the ions energy distribution in equilibrium. We provide analytic expressions and numerical simulations of the ions energy distribution, spatial profile and cooling rates for these different regimes. Based on these findings, a method for actively decreasing the ions energy by reducing the spatial expansion of the buffer gas arises (Forced Sympathetic Cooling).
We present a quantum logic scheme to detect atomic and molecular ions in different states of angular momentum based on their magnetic $g$-factors. The state-dependent magnetic $g$-factors mean that electronic, rotational or hyperfine states may be distinguished by their Zeeman splittings in a given magnetic field. Driving motional sidebands of a chosen Zeeman splitting enables reading out the corresponding state of angular momentum with an auxillary logic ion. As a proof-of-principle demonstration, we show that we can detect the ground electronic state of a ${^{174}}$Yb$^+$ ion using ${^{171}}$Yb$^+$ as the logic ion. Further, we can distinguish between the ${^{174}}$Yb$^+$ ion being in its ground electronic state versus the metastable ${^{2}}D_{3/2}$ state. We discuss the suitability of this scheme for the detection of rotational states in molecular ions.
Controlling physical systems and their dynamics on the level of individual quanta propels both fundamental science and quantum technologies. Trapped atomic and molecular systems, neutral and charged, are at the forefront of quantum science. Their extraordinary level of control is evidenced by numerous applications in quantum information processing and quantum metrology. Studying the long-range interactions between these systems when combined in a hybrid atom-ion trap has lead to landmark results. Reaching the ultracold regime, however, where quantum mechanics dominates the interaction, e.g., giving access to controllable scattering resonances, has been elusive so far. Here we demonstrate Feshbach resonances between ions and atoms, using magnetically tunable interactions between $^{138}$Ba$^{+}$ ions and $^{6}$Li atoms. We tune the experimental parameters to probe different interaction processes - first, enhancing three-body reactions and the related losses to identify the resonances, then making two-body interactions dominant to investigate the ions sympathetic cooling in the ultracold atomic bath. Our results provide deeper insights into atom-ion interactions, giving access to complex many-body systems and applications in experimental quantum simulation.
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