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Register a new userUltraviolet and visible range plasmonics of a topological insulator
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The development of metamaterials, data processing circuits and sensors for the visible and UV parts of the spectrum is hampered by the lack of low-loss media supporting plasmonic excitations and drives the intense search for plasmonic materials beyond noble metals. By studying plasmonic nanostructures fabricated on the surface of topological insulator $mbox{Bi}_{1.5}mbox{Sb}_{0.5}mbox{Te}_{1.8}mbox{Se}_{1.2}$ we found that it is orders of magnitude better plasmonic material than gold and silver in the blue-UV range. Metamaterial fabricated from $mbox{Bi}_{1.5}mbox{Sb}_{0.5}mbox{Te}_{1.8}mbox{Se}_{1.2}$ show plasmonic resonances from 350 nm to 550 nm while surface gratings exhibit cathodoluminescent peaks from 230 nm to 1050 nm. The negative permittivity underpinning plasmonic response is attributed to the combination of bulk interband transitions and surface contribution of the topologically protected states. The importance of our result is in the identification of new mechanisms of negative permittivity in semiconductors where visible-range plasmonics can be directly integrated with electronics.
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Although the first lasers invented operated in the visible, the first on-chip devices were optimized for near-infrared (IR) performance driven by demand in telecommunications. However, as the applications of integrated photonics has broadened, the wavelength demand has as well, and we are now returning to the visible (Vis) and pushing into the ultraviolet (UV). This shift has required innovations in device design and in materials as well as leveraging nonlinear behavior to reach these wavelengths. This review discusses the key nonlinear phenomena that can be used as well as presents several emerging material systems and devices that have reached the UV-Vis wavelength range.
Microlaser with multiple lasing bands is critical in various applications, such as full-colour display, optical communications and computing. Here, we propose a simple and efficient method for homogeneously doping rare earth elements into a silica whispering-gallery-mode microcavity. By this method, we demonstrate simultaneous and stable lasing covering ultraviolet, visible and near-infrared bands in an ultrahigh-Q (exceeding 108) Er-Yb co-doped silica microsphere under room temperature and continuous-wave pump for the first time. The lasing thresholds of the 380, 410, 450, 560, 660, 800, 1080 and 1550 nm-bands are estimated to be 380, 150, 2.5, 12, 0.17, 1.7, 10 and 38 {mu}W, respectively, where the lasing in the 380, 410 and 450 nm-bands by Er element have not been separately demonstrated under room temperature and continuous-wave pump until this work. This ultrahigh-Q doped microcavity is an excellent platform for high-performance multi-band microlasers, ultrahigh-precise sensors, optical memories and cavity-enhanced light-matter interaction studies.
Wavelength-sized microdisk resonators were fabricated on a single crystalline 4H-silicon-carbide-oninsulator platform (4H-SiCOI). By carrying out microphotoluminescence measurements at room temperature, we show that the microdisk resonators support whispering-gallery modes (WGMs) with quality factors up to $5.25 times 10^3$ and mode volumes down to $2.69 times(lambda /n)^3$ at the visible and near-infrared wavelengths. Moreover, the demonstrated wavelength-sized microdisk resonators exhibit WGMs whose resonant wavelengths compatible with the zero-phonon lines of spin defects in 4H-SiCOI, making them a promising candidate for applications in cavity quantum electrodynamics and integrated quantum photonic circuits.
We demonstrate a passive down-conversion imaging system that converts broadband ultraviolet light to narrow-band green light while preserving the directionality of rays, and thus enabling direct down-conversion imaging. At the same time our system has high transparency in the visible, enabling superimposed visible and ultraviolet imaging. The frequency conversion is performed by a subwavelength-thickness transparent downconverter based on highly efficient CsPbBr3 nanocrystals incorporated into the focal plane of a simple telescope or relay-lens geometry. The resulting imaging performance of this down-conversion system approaches the diffraction limit. This demonstration sets the stage for the incorporation of other high-efficiency perovskite nanocrystal materials to enable passive multi-frequency conversion imaging systems.
Ultraviolet (UV) plasmonics aims at combining the strong absorption bands of molecules in the UV range with the intense electromagnetic fields of plasmonic nanostructures to promote surface-enhanced spectroscopy and catalysis. Currently, aluminum is the most widely used metal for UV plasmonics, and is generally assumed to be remarkably stable thanks to its natural alumina layer passivating the metal surface. However, we find here that under 266 nm UV illumination, aluminum can undergo a dramatic photocorrosion in water within a few tens of seconds and even at low average UV powers. This aluminum instability in water environments critically limits the UV plasmonics applications. We show that the aluminum photocorrosion is related to the nonlinear absorption by water in the UV range leading to the production of hydroxyl radicals. Different corrosion protection approaches are tested using scavengers for reactive oxygen species and polymer layers deposited on top of the aluminum structures. Using optimized protection, we achieve a ten-fold increase in the available UV power range leading to no visible photocorrosion effects. This technique is crucial to achieve stable use of aluminum nanostructures for UV plasmonics in aqueous solutions.
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