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Register a new userNonlinear nanophotonic devices in the Ultraviolet to Visible wavelength range
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Although the first lasers invented operated in the visible, the first on-chip devices were optimized for near-infrared (IR) performance driven by demand in telecommunications. However, as the applications of integrated photonics has broadened, the wavelength demand has as well, and we are now returning to the visible (Vis) and pushing into the ultraviolet (UV). This shift has required innovations in device design and in materials as well as leveraging nonlinear behavior to reach these wavelengths. This review discusses the key nonlinear phenomena that can be used as well as presents several emerging material systems and devices that have reached the UV-Vis wavelength range.
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The development of inverse design, where computational optimization techniques are used to design devices based on certain specifications, has led to the discovery of many compact, non-intuitive structures with superior performance. Among various methods, large-scale, gradient-based optimization techniques have been one of the most important ways to design a structure containing a vast number of degrees of freedom. These techniques are made possible by the adjoint method, in which the gradient of an objective function with respect to all design degrees of freedom can be computed using only two full-field simulations. However, this approach has so far mostly been applied to linear photonic devices. Here, we present an extension of this method to modeling nonlinear devices in the frequency domain, with the nonlinear response directly included in the gradient computation. As illustrations, we use the method to devise compact photonic switches in a Kerr nonlinear material, in which low-power and high-power pulses are routed in different directions. Our technique may lead to the development of novel compact nonlinear photonic devices.
We present a digitized adjoint method for realizing efficient inverse design of digital subwavelength nanophotonic devices. We design a single-mode 3-dB power divider and a dual-mode demultiplexer to demonstrate the digitized adjoint method for single-object and dual-object optimizations, respectively. The optimization comprises three stages, a first stage of continuous variation for an analog pattern, a second stage of forced permittivity biasing for a quasi-digital pattern, and a third stage for a multi-level digital pattern. Compared with conventional brute-force method, the proposed digitized adjoint method can improve the design efficiency by about 5 times, and the performance optimization can reach approximately the same level using the ternary pattern. The digitized adjoint method takes the advantages of adjoint sensitivity analysis and digital subwavelength structure and creates a new way for efficient and high-performance design of compact digital subwavelength nanophotonic devices. This method could overcome the efficiency bottleneck of the brute-force method that is restricted by the number of pixels of a digital pattern and improve the device performance by extending a conventional binary pattern to a multi-level one, which may be attractive for inverse design of large-scale digital nanophotonic devices.
We demonstrate a passive down-conversion imaging system that converts broadband ultraviolet light to narrow-band green light while preserving the directionality of rays, and thus enabling direct down-conversion imaging. At the same time our system has high transparency in the visible, enabling superimposed visible and ultraviolet imaging. The frequency conversion is performed by a subwavelength-thickness transparent downconverter based on highly efficient CsPbBr3 nanocrystals incorporated into the focal plane of a simple telescope or relay-lens geometry. The resulting imaging performance of this down-conversion system approaches the diffraction limit. This demonstration sets the stage for the incorporation of other high-efficiency perovskite nanocrystal materials to enable passive multi-frequency conversion imaging systems.
The development of metamaterials, data processing circuits and sensors for the visible and UV parts of the spectrum is hampered by the lack of low-loss media supporting plasmonic excitations and drives the intense search for plasmonic materials beyond noble metals. By studying plasmonic nanostructures fabricated on the surface of topological insulator $mbox{Bi}_{1.5}mbox{Sb}_{0.5}mbox{Te}_{1.8}mbox{Se}_{1.2}$ we found that it is orders of magnitude better plasmonic material than gold and silver in the blue-UV range. Metamaterial fabricated from $mbox{Bi}_{1.5}mbox{Sb}_{0.5}mbox{Te}_{1.8}mbox{Se}_{1.2}$ show plasmonic resonances from 350 nm to 550 nm while surface gratings exhibit cathodoluminescent peaks from 230 nm to 1050 nm. The negative permittivity underpinning plasmonic response is attributed to the combination of bulk interband transitions and surface contribution of the topologically protected states. The importance of our result is in the identification of new mechanisms of negative permittivity in semiconductors where visible-range plasmonics can be directly integrated with electronics.
Over the past decade, remarkable advances have been realized in chip-based nonlinear photonic devices for classical and quantum applications in the near- and mid-infrared regimes. However, few demonstrations have been realized in the visible and near-visible regimes, primarily due to the large normal material group-velocity dispersion (GVD) that makes it challenging to phase match third-order parametric processes. In this paper, we show that exploiting dispersion engineering of higher-order waveguide modes provides waveguide dispersion that allows for small or anomalous GVD in the visible and near-visible regimes and phase matching of four-wave mixing processes. We illustrate the power of this concept by demonstrating in silicon nitride microresonators a near-visible modelocked Kerr frequency comb and a narrow-band photon-pair source compatible with Rb transitions. These realizations extend applications of nonlinear photonics towards the visible and near-visible regimes for applications in time and frequency metrology, spectral calibration, quantum information, and biomedical applications.
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