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Register a new userMid-IR frequency measurement using an optical frequency comb and a long-distance remote frequency reference
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Authors
Bruno Chanteau
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We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an ultrastable 1.55 $mu$m frequency reference signal, transferred from LNE-SYRTE to LPL through an optical link. We are now progressing towards the stabilization of the mid-IR laser via the frequency comb and the extension of this technique to quantum cascade lasers. Such a development is very challenging for ultrahigh resolution molecular spectroscopy and fundamental tests of physics with molecules.
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We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 mum) and thus covering much of the infrared fingerprint molecular vibration region. It is based on nonlinear frequency conversion in GaSe using a compact commercial 100-fs-pulsed Er fiber laser system providing two amplified near-infrared beams, one of them broadened by a nonlinear optical fiber. The resulting collimated mid-infrared continuum beam of 1 mW quasi-cw power represents a coherent infrared frequency comb with zero carrier-envelope phase, containing about 500,000 modes that are exact multiples of the pulse repetition rate of 40 MHz. The beams diffraction-limited performance enables long-distance spectroscopic probing as well as maximal focusability for classical and ultraresolving near-field microscopies. Applications are foreseen also in studies of transient chemical phenomena even at ultrafast pump-probe scale, and in high-resolution gas spectroscopy for e.g. breath analysis.
We describe a measurement of the frequency of the 2S1/2(F = 0) - 2D3/2(F = 2) transition of 171Yb+ at the wavelength 436 nm (frequency 688 THz), using a single Yb+ ion confined in a Paul trap and two caesium fountains as references. In one of the fountains, the frequency of the microwave oscillator that interrogates the caesium atoms is stabilized by the laser that excites the Yb+ reference transition with a linewidth in the hertz range. The stability is transferred to the microwave oscillator with the use of a fiber laser based optical frequency comb generator that also provides the frequency conversion for the absolute frequency measurement. The frequency comb generator is configured as a transfer oscillator so that fluctuations of the pulse repetition rate and of the carrier offset frequency do not degrade the stability of the frequency conversion. The phase noise level of the generated ultrastable microwave signal is comparable to that of a cryogenic sapphire oscillator. For fountain operation with optical molasses loaded from a laser cooled atomic beam source, we obtain a stability corresponding to a fractional Allan deviation of $4.1times 10^{-14} (tau/text{s})^{-1/2}$. With the molasses loaded from thermal vapor and an averaging time of 65 h, we measure the frequency of the Yb+ transition with a relative statistical uncertainty of $2.8times10^{-16}$ and a systematic uncertainty of $5.9times10^{-16}$. The frequency was also simultaneously measured with the second fountain that uses a quartz-based interrogation oscillator. The unperturbed frequency of the Yb+ transition is realized with an uncertainty of $1.1times10^{-16}$ that mainly results from the uncertainty of the blackbody shift at the operating temperature near 300 K. The transition frequency of 688 358 979 309 307.82(36) Hz, measured with the two fountains, is in good agreement with previous results.
Measuring the spectral properties of an optical frequency comb is among the most fundamental tasks of precision metrology. In contrast to general single-parameter measurement schemes, we demonstrate here single shot multiparameter estimation at and beyond the standard quantum limit. The mean energy and the central frequency of ultrafast pulses are simultaneously determined with a multi-pixel-spectrally-resolved (MPSR) apparatus, without changing the photonics architecture. Moreover, using a quantum frequency comb that consists of multiple squeezed states in a family of Hermite-Gaussian spectral/temporal modes, the signal-to-noise ratios of the mean energy and the central frequency measurements surpass the shot-noise limit by around 19% and 15%, respectively. Combining our multi-pixel detection scheme and the intrinsic multimode quantum resource could find applications in ultrafast quantum metrology and multimode quantum information processing.
The absolute frequency of the $^{87}{rm Sr}$ lattice clock transition was evaluated with an uncertainty of $1.1times 10^{-15}$ using a frequency link to the international atomic time (TAI). The frequency uncertainty of a hydrogen maser used as a transfer oscillator was reduced by homogeneously distributed intermittent measurement over a five-day grid of TAI. Three sets of four or five days measurements as well as systematic uncertainty of the clock at $8.6times 10^{-17}$ have resulted in an absolute frequency of $^{87}{rm Sr} {}^1S_0 - {}^3P_0$ clock transition to be 429 228 004 229 872.85 (47) Hz.
Using a turn-key Ti:sapphire femtosecond laser frequency comb, an off-the-shelf supercontinuum device, and Fabry-Perot mode filters, we report the generation of a 16 GHz frequency comb spanning a 90 nm band about a center wavelength of 566 nm. The light from this astro-comb is used to calibrate the HARPS-N astrophysical spectrograph for precision radial velocity measurements. The comb-calibrated spectrograph achieves a stability of $sim$ 1 cm/s within half an hour of averaging time. We also use the astro-comb as a reference for measurements of solar spectra obtained with a compact telescope, and as a tool to study intrapixel sensitivity variations on the CCD of the spectrograph.
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