No Arabic abstract
We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 mum) and thus covering much of the infrared fingerprint molecular vibration region. It is based on nonlinear frequency conversion in GaSe using a compact commercial 100-fs-pulsed Er fiber laser system providing two amplified near-infrared beams, one of them broadened by a nonlinear optical fiber. The resulting collimated mid-infrared continuum beam of 1 mW quasi-cw power represents a coherent infrared frequency comb with zero carrier-envelope phase, containing about 500,000 modes that are exact multiples of the pulse repetition rate of 40 MHz. The beams diffraction-limited performance enables long-distance spectroscopic probing as well as maximal focusability for classical and ultraresolving near-field microscopies. Applications are foreseen also in studies of transient chemical phenomena even at ultrafast pump-probe scale, and in high-resolution gas spectroscopy for e.g. breath analysis.
Implementing optical-frequency combs with integrated photonics will enable wider use of precision timing signals.Here, we explore the generation of an octave-span, Kerr-microresonator frequency comb, using hybrid integration ofan InP distributed-feedback laser and a SiN photonic-integrated circuit. We demonstrate electrically pumped and fiber-packaged prototype systems, enabled by self-injection locking. This direct integration of a laser and a microresonatorcircuit without previously used intervening elements, like optical modulators and isolators, necessitates understand-ing self-injection-locking dynamics with octave-span Kerr solitons. In particular, system architectures must adjust tothe strong coupling of microresonator back-scattering and laser-microresonator frequency detuning that we uncoverhere. Our work illustrates critical considerations towards realizing a self-referenced frequency comb with integratedphotonics.
We present a laser frequency comb based upon a 250 MHz mode-locked erbium-doped fiber laser that spans more than 300 terahertz of bandwidth, from 660 nm to 2000 nm. The system generates 1.2 nJ, 70 fs pulses at 1050 nm by amplifying the 1580 nm laser light in Er:fiber, followed by nonlinear broadening to 1050 nm and amplification in Yb:fiber. Extension of the frequency comb into the visible is achieved by supercontinuum generation from the 1050 nm light. Comb coherence is verified with cascaded f-2f interferometry and comparison to a frequency stabilized laser.
We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an ultrastable 1.55 $mu$m frequency reference signal, transferred from LNE-SYRTE to LPL through an optical link. We are now progressing towards the stabilization of the mid-IR laser via the frequency comb and the extension of this technique to quantum cascade lasers. Such a development is very challenging for ultrahigh resolution molecular spectroscopy and fundamental tests of physics with molecules.
We demonstrate the generation of a low-noise, octave-spanning mid-infrared supercontinuum from 1700 to 4800 nm by injecting femtosecond pulses into the normal dispersion regime of a multimode step-index chalcogenide fiber with 100 $mu$m core diameter. We conduct a systematic study of the intensity noise across the supercontinuum spectrum and show that the initial fluctuations of the pump laser are at most amplified by a factor of three. We also perform a comparison with the noise characteristics of an octave-spanning supercontinuum generated in the anomalous dispersion regime of a multimode fluoride fiber with similar core size and show that the all-normal dispersion supercontinuum in the multimode chalcogenide fiber has superior noise characteristics. Our results open up novel perspective for many practical applications such as long-distance remote sensing where high power and low noise are paramount.
We have experimentally demonstrated how two beams of light separated by an octave in frequency can become entangled after their interaction in a second-order nonlinear medium. The entangler consisted of a nonlinear crystal placed within an optical resonator that was strongly driven by coherent light at the fundamental and second-harmonic wavelengths. An inter-conversion between the fields created quantum correlations in the amplitude and phase quadratures, which were measured by two independent homodyne detectors. Analysis of the resulting correlation matrix revealed a wavefunction inseparability of 0.74(1) < 1 thereby satisfying the criterion of entanglement.