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Register a new userQuantum efficiency of technical metal photocathodes under laser irradiation of various wavelength
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Quantum efficiency studies for various wavelength and various technical metal surfaces were carried out in a dedicated unbaked vacuum chamber. Copper, magnesium, aluminium and aluminium-lithium photocathodes were irradiated by two different high power, high repetition rate, laser systems. We have observed an emission of electrons for photon energy below the work function of the material. This is explained by multiple photon absorption at the photocathode. We have not observed any degradation of the QE for those materials, but an improvement when irradiating them over a long period of time. This is contrary to observations made in RF photoguns.
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We report quantum efficiency (QE) enhancements in accelerator technology relevant antimonide photocathodes (K2CsSb) by interfacing them with atomically thin two-dimensional (2D) crystal layers. The enhancement occurs in a reflection mode, when a 2D crystal is placed in between the photocathodes and optically reflective substrates. Specifically, the peak QE at 405 nm (3.1 eV) increases by a relative 10 percent, while the long wavelength response at 633 nm (2.0 eV) increases by a relative 36 percent on average and up to 80 percent at localized hot spot regions when photocathodes are deposited onto graphene coated stainless steel. There is a similar effect for photocathodes deposited on hexagonal boron nitride monolayer coatings using nickel substrates. The enhancement does not occur when reflective substrates are replaced with optically transparent sapphire. Optical transmission, X-ray diffraction (XRD) and X-ray fluorescence (XRF) revealed that thickness, crystal orientation, quality and elemental stoichiometry of photocathodes do not appreciably change due to 2D crystal coatings. These results suggest optical interactions are responsible for the QE enhancements when 2D crystal sublayers are present on reflective substrates, and provide a pathway toward a simple method of QE enhancement in semiconductor photocathodes by an atomically thin 2D crystal on substrates.
Aspects of the preparation process and performance degradation are two major problems of photocathodes. The lack of a means for dynamic quantum efficiency measurements results in the inability to observe the inhomogeneity of the cathode surface by fine structural analysis and in real time.Here we present a simple and scalable technique for in situ real-time quantum efficiency diagnosis. An incoherent light source provides uniform illumination on the cathode surface, and solenoid magnets are used as lens for focusing and imaging the emitted electron beam on a downstream scintillator screen, which converts the quantum efficiency information into fluorescence intensity distribution. The microscopic discontinuity and the dynamic changes of the quantum efficiency of a gallium arsenide photocathode are observed at a resolution of a few microns. An unexpected uneven decrease of the quantum efficiency is also recorded. The work demonstrates a new observation method for photoemission materials research.
A detailed study of the circular photogalvanic effect (CPGE) in SiGe structures is presented. It is shown that the CPGE becomes possible due to the built-in asymmetry of quantum wells (QWs) in compositionally stepped samples and in asymmetrically doped structures. The photocurrent arises due to optical spin orientation of free carriers in QWs with spin splitting in k-space. It is shown that the effect can be applied to probe the macroscopic in-plane symmetry of low dimensional structures and allowing to conclude on Rashba or Dresselhaus terms in the Hamiltonian.
Future linear colliders will require high levels of performance from their electron sources. A group at SLAC has recently tested a structure that substantially exceeds current collider polarized electron source pulse-profile requirements.
High irradiance lasers incident on metal surfaces create a complex, dynamic process through which the metal can rapidly change from highly reflective to strongly absorbing. Absolute knowledge of this process underpins important industrial laser processes like laser welding, cutting, and metal additive manufacturing. Determining the time-dependent absorptance of the laser light by a material is important, not only for gaining a fundamental understanding of the light-matter interaction, but also for improving process design in manufacturing. Measurements of the dynamic optical absorptance are notoriously difficult due to the rapidly changing nature of the absorbing medium. This data is also of vital importance to process modelers whose complex simulations need reliable, accurate input data; yet, there is very little available. In this work, we measure the time-dependent, reflected light during a 10 ms laser spot weld using an integrating sphere apparatus. From this, we calculate the dynamic absorptance for 1070 nm wavelength light incident on 316L stainless steel. The time resolution of our experiment (< 1 us) allows for the determination of the precise conditions under which several important physical phenomena occur, such as melt and keyhole formation. The average absorptances determined optically were compared to calorimetrically-determined values, and it was found that the calorimeter severely underestimated the absorbed energy due to mass lost during the spot weld. Weld nugget cross-sections are also presented in order to verify our interpretation of the optical results, as well as provide experimental data for weld model validation.
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