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An $it{ab ,, initio}$ based fully microscopic approach is applied to study the nonlinear optical response of bulk Tellurium. The structural and electronic properties are calculated from first principles using the shLDA-1/2 method within density functional theory. The resulting bandstructure and dipole matrix elements serve as input for the quantum mechanical evaluation of the anisotropic linear optical absorption spectra yielding results in excellent agreement with published experimental data. Assuming quasi-equilibrium carrier distributions in the conduction and valence bands, absorption/gain and spontaneous emission spectra are computed from the semiconductor Bloch and luminescence equations. For ultrafast intense off-resonant excitation, the generation of high-harmonics is evaluated and the emission spectra are calculated for samples of different thickness.
Three-color coherent anti-Stokes Raman scattering represents non-degenerate four wave mixing process that includes both a non-resonant and resonant processes, the contributions of which depend on how the molecular vibrational modes are being excited
A convenient for practical use new theoretical approach describing a nonlinear frequency response of the multi-resonant nonlinear ring cavities (RC) to an intense monochromatic wave action is developed. The approach closely relates the many-valuednes
The theory of incoherent nuclear resonant scattering of synchrotron radiation accompanied by absorption or emission of phonons in a crystal lattice is developed. The theory is based on the Maxwells equations and time-dependent quantum mechanics under
Optical cavities are a cornerstone of photonics. They are indispensable in lasers, optical filters, optical combs and clocks, in quantum physics, and have enabled the detection of gravitational waves. Cavities transmit light only at discrete resonant
Coherent perfect absorption (CPA) refers to interferometrically induced complete absorption of incident light by a partial absorber independently of its intrinsic absorption (which may be vanishingly small) or its thickness. CPA is typically realized