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We demonstrate Bragg diffraction of the antibiotic ciprofloxacin and the dye molecule phthalocyanine at a thick optical grating. The observed patterns show a single dominant diffraction order with the expected dependence on the incidence angle as well as oscillating population transfer between the undiffracted and diffracted beams. We achieve an equal-amplitude splitting of $14 hbar k$ (photon momenta) and maximum momentum transfer of $18 hbar k$. This paves the way for efficient, large-momentum beam splitters and mirrors for hot and complex molecules.
The use of retro-reflection in light-pulse atom interferometry under microgravity conditions naturally leads to a double-diffraction scheme. The two pairs of counterpropagating beams induce simultaneously transitions with opposite momentum transfer t
Bragg diffraction of an atomic wave packet in a retroreflective geometry with two counterpropagating optical lattices exhibits a light shift induced phase. We show that the temporal shape of the light pulse determines the behavior of this phase shift
We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a double kick scheme) or
For conventional imaging, shaking of the imaging system or the target leads to the degradation of imaging resolution. In this work, the influence of the targets shaking to fourier-transform ghost diffraction (FGD) is investigated. The analytical resu
Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and molecular