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تسجيل مستخدم جديدBright, polarization-tunable high repetition rate extreme ultraviolet beamline for coincidence electron-ion imaging
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After decades of supremacy of the Titanium:Sapphire technology, Ytterbium-based high-order harmonic sources are emerging as an interesting alternative for experiments requiring high flux of ultrashort extreme ultraviolet (XUV) radiation. In this article we describe a versatile experimental setup delivering XUV photons in the 10-50 eV range. The use of cascaded high-harmonic generation enables us to reach 1.8 mW of average power at 18 eV. Several spectral focusing schemes are presented, to select either a single harmonic or group of high-harmonics and thus an attosecond pulse train. In the perspective of circular dichroism experiments, we produce highly elliptical XUV radiation using resonant elliptical high-harmonic generation, and circularly polarized XUV by bichromatic bicircular high-harmonic generation. As a proof of principle experiment, we focus the XUV beam in a coincidence electron-ion imaging spectrometer, where we measure the photoelectron momentum angular distributions of xenon monomers and dimers.
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High harmonic generation (HHG) enables coherent extreme-ultraviolet (XUV) radiation with ultra-short pulse duration in a table-top setup. This has already enabled a plethora of applications. Nearly all of these applications would benefit from a high
photon flux to increase the signal-to-noise ratio and decrease measurement times. In addition, shortest pulses are desired to investigate fastest dynamics in fields as diverse as physics, biology, chemistry and material sciences. In this work, the up-to-date most powerful table-top XUV source with 12.9 mW in a single harmonic line at 26.5 eV is demonstrated via HHG of a frequency-doubled and post-compressed fibre laser. At the same time sub-6 fs XUV pulse duration allows accessing ultrafast dynamics with an order of magnitude higher photon flux than previously demonstrated. This concept will greatly advance and facilitate applications of XUV radiation in science and technology and enable photon-hungry ultrafast studies.
Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates, $f_{rep}lesssim$100
kHz, where phase-matched frequency conversion into the XUV is readily achieved. However, there are many applications that demand the improved counting statistics or frequency-comb precision afforded by operation at high repetition rates, $f_{rep}$ > 10 MHz. Unfortunately, at such high $f_{rep}$, phase matching is prevented by the accumulated steady-state plasma in the generation volume, setting stringent limitations on the XUV average power. Here, we use gas mixtures at high temperatures as the generation medium to increase the translational velocity of the gas, thereby reducing the steady-state plasma in the laser focus. This allows phase-matched XUV emission inside a femtosecond enhancement cavity at a repetition rate of 77 MHz, enabling a record generated power of $sim$2 mW in a single harmonic order. This power scaling opens up many demanding applications, including XUV frequency-comb spectroscopy of few-electron atoms and ions for precision tests of fundamental physical laws and constants.
The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated attosecond
pulses, they continue to be a unique tool enabling the observation and control of electron dynamics in atoms, molecules and solids. It has long been identified that an increase in the repetition rate of attosecond light sources is necessary for many applications in atomic and molecular physics, surface science, and imaging. Although high harmonic generation (HHG) at repetition rates exceeding 100 kHz, showing a continuum in the cut-off region of the XUV spectrum was already demonstrated in 2013, the number of photons per pulse was insufficient to perform pulse characterisation via attosecond streaking, let alone to perform a pump-probe experiment. Here we report on the generation and full characterisation of XUV attosecond pulses via HHG driven by near-single-cycle pulses at a repetition rate of 100 kHz. The high number of 10^6 XUV photons per pulse on target enables attosecond electron streaking experiments through which the XUV pulses are determined to consist of a dominant single attosecond pulse. These results open the door for attosecond pump-probe spectroscopy studies at a repetition rate one or two orders of magnitude above current implementations.
We propose and numerically validate an all-optical scheme to generate optical pulse trains with varying temporal pulse-to-pulse delay and pulse duration. Applying a temporal sinusoidal phase modulation followed by a shaping of the spectral phase enab
les us to maintain high-quality Gaussian temporal profiles.
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Alexey Andrianov
, Arkady Kim (Institute of Applied Physics of then Russian Academy of Sciences
, Nizhny Novgorod
2019
We present the first direct observation of the bound state of multiple dissipative optical solitons in which bond length and bond strength can be individually controlled in a broad range in a regular manner. We have observed experimentally a new type
of stable and extremely elastic soliton crystals that can be stretched and compressed many times conserving their structure by adjusting the bond properties in real time in a specially designed passively mode-locked fiber laser incorporating highly asymmetric tunable Mach-Zehnder interferometer. The temporal structure and dynamics of the generated soliton crystals have been studied using an asynchronous optical sampling system with picosecond resolution. We demonstrated that stable and robust soliton crystal can be formed by two types of primitive structures: single dissipative solitons, and(or) pairs of dissipative soliton and pulse with lower amplitude. Continuous stretching and compression of a soliton crystal with extraordinary high ratio of more than 30 has been demonstrated with a smallest recorded separation between pulses as low as 5 ps corresponding to an effective repetition frequency of 200 GHz. Collective pulse dynamics, including soliton crystal self-assembling, cracking and transformation of crystals comprising pulse pairs to the crystals of similar pulses has been observed experimentally.
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