اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدTheoretical study of ArH+ dissociative recombination and electron-impact vibrational excitation
101
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Cross sections are presented for dissociative recombination and electron-impact vibrational excitation of the ArH+ molecular ion at electron energies appropriate for the interstellar environment. The R-matrix method is employed to determine the molecular structure data, i.e. the position and width of the resonance states. The cross sections and the corresponding Maxwellian rate coefficients are computed using a method based on the Multichannel Quantum Defect Theory. The main result of the paper is the very low dissociative recombination rate found at temperatures below 1000K. This is in agreement with the previous upper limit measurement in merged beams and offers a realistic explanation to the presence of ArH+ in exotic interstellar conditions.
قيم البحث
اقرأ أيضاً
For understanding carbon erosion and redeposition in nuclear fusion devices, it is important to understand the transport and chemical break-up of hydrocarbon molecules in edge plasmas, often diagnosed by emission of the CH A^2Delta - X^2Pi Gero band
around 430 nm. The CH A-level can be excited either by electron-impact or by dissociative recombination (D.R.) of hydrocarbon ions. These processes were included in the 3D Monte Carlo impurity transport code ERO. A series of methane injection experiments was performed in the high-density, low-temperature linear plasma generator Pilot-PSI, and simulated emission intensity profiles were benchmarked against these experiments. It was confirmed that excitation by D.R. dominates at T_e < 1.5 eV. The results indicate that the fraction of D.R. events that lead to a CH radical in the A-level and consequent photon emission is at least 10%. Additionally, quenching of the excited CH radicals by electron impact de-excitation was included in the modeling. This quenching is shown to be significant: depending on the electron density, it reduces the effective CH emission by a factor of 1.4 at n_e=1.3*10^20 m^-3, to 2.8 at n_e=9.3*10^20 m^-3. Its inclusion significantly improved agreement between experiment and modeling.
A theoretical investigation of the dissociative excitation by electron impact on the NO molecule is presented, aiming to make up for the lack of data for this process in the literature. A full set of vibrationally-resolved cross sections and correspo
nding rate coefficients are calculated using the Local-Complex-Potential approach and five resonant states of NO^-.
Emission and absorption features from C-like ions serve as temperature and density diagnostics of astrophysical plasmas. $R$-matrix electron-impact excitation data sets for C-like ions in the literature merely cover a few ions, and often only for the
ground configuration. Our goal is to obtain level-resolved effective collision strength over a wide temperature range for C-like ions from ion{N}{II} to ion{Kr}{XXXI} (i.e., N$^{+}$ to Kr$^{30+}$) with a systematic set of $R$-matrix calculations. We also aim to assess their accuracy. For each ion, we included a total of 590 fine-structure levels in both the configuration interaction target and close-coupling collision expansion. These levels arise from 24 configurations $2l^3 nl^{prime}$ with $n=2-4$, $l=0-1$, and $l^{prime}=0-3$ plus the three configurations $2s^22p5l$ with $l=0-2$. The AUTOSTRUCTURE code was used to calculate the target structure. Additionally, the $R$-matrix intermediate coupling frame transformation method was used to calculate the collision strengths. We compare the present results of selected ions with archival databases and results in the literature. The comparison covers energy levels, transition rates, and effective collision strengths. We illustrate the impact of using the present results on an ion{Ar}{xiii} density diagnostic for the solar corona. The electron-impact excitation data is archived according to the Atomic Data and Analysis Structure (ADAS) data class adf04 and will be available in OPEN-ADAS. The data will be incorporated into spectral codes, such as CHIANTI and SPEX, for plasma diagnostics.
Spectral lines from N-like ions can be used to measure the temperature and density of various types of astrophysical plasmas. The atomic databases of astrophysical plasma modelling codes still have room for improvement in their electron-impact excita
tion data sets for N-like ions, especially $R$-matrix data. This is particularly relevant for future observatories (e.g. Arcus) which will host high-resolution spectrometers. We aim to obtain level-resolved effective collision strengths for all transitions up to $nl=5d$ over a wide range of temperatures for N-like ions from O II to Zn XXIV (i.e., O$^{+}$ to Zn$^{23+}$) and to assess the accuracy of the present work. We also examine the impact of our new data on plasma diagnostics by modelling solar observations with CHIANTI. We have carried-out systematic $R$-matrix calculations for N-like ions which included 725 fine-structure target levels in both the configuration interaction target and close-coupling collision expansions. The $R$-matrix intermediate coupling frame transformation method was used to calculate the collision strengths, while the AUTOSTRUCTURE code was used for the atomic structures. We compare the present results for selected ions with those in archival databases and the literature. The comparison covers energy levels, oscillator strengths, and effective collision strengths. We show examples of improved plasma diagnostics when compared to CHIANTI models which use only distorted wave data as well as some which use previous $R$-matrix data. The electron-impact excitation data are archived according to the Atomic Data and Analysis Structure (ADAS) data class it adf04 and will be available in OPEN-ADAS. The data can be used to improve the atomic databases for astrophysical plasma diagnostics.
The long-standing difference in chemical abundances determined from optical recombination lines and collisionally excited lines raises questions about our understanding of atomic physics, as well as the assumptions made when determining physical cond
itions and chemical abundances in astrophysical nebulae. Here, we study the recombination contribution of [O III] 4363 and the validity of the line ratio [O III] 4363/4959 as a temperature diagnostic in planetary nebulae with a high abundance discrepancy. We derive a fit for the recombination coefficient of [O III] 4363 that takes into account the radiative and dielectronic recombinations, for electron temperatures from 200 to 30,000 K. We estimate the recombination contribution of [O III] 4363 for the planetary nebulae Abell 46 and NGC 6778 by subtracting the collisional contribution from the total observed flux. We find that the spatial distribution for the estimated recombination contribution in [O III] 4363 follows that of the O II 4649 recombination line, both peaking in the central regions of the nebula, especially in the case of Abell 46 which has a much higher abundance discrepancy. The estimated recombination contribution reaches up to 70% and 40% of the total [O III] 4363 observed flux, for Abell 46 and NGC 6778, respectively.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
