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تسجيل مستخدم جديدSearch for cosmic dark matter by means of ultra high purity NaI(Tl) scintillator
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The dark matter search project by means of ultra high purity NaI(Tl) scintillator is now underdevelopment. An array of large volume NaI(Tl) detectors whose volume is 12.7 cm$phitimes$12.7 cm is applied to search for dark matter signal. To remove radioactive impurities in NaI(Tl) crystal is one of the most important task to find small number of dark matter signals. We have developed high purity NaI(Tl) crystal which contains small amounts of radioactive impurities, $<4$ ppb of $^{nat}$K, 0.3 ppt of Th chain, 58 $mu$Bq/kg of $^{226}$Ra and 30 $mu$Bq/kg of $^{210}$Pb. Future prospects to search for dark matter by means of a large volume and high purity NaI(Tl) scintillator is discussed.
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A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl)
crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $mu$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector module will be reported in this article.
A high purity and large volume NaI(Tl) scintillator was developed to search for cosmic dark matter. The required densities of radioactive impurities (RIs) such as U-chain, Th-chain are less than a few ppt to establish high sensitivity to dark matter.
The impurity of RIs were effectively reduced by selecting raw materials of crucible and by performing chemical reduction of lead ion in NaI raw powder. The impurity of $^{226}$Ra was reduced less than 100 $mu$Bq/kg in NaI(Tl) crystal. It should be remarked that the impurity of $^{210}$Pb, which is difficult to reduce, is effectively reduced by chemical processing of NaI raw powder down to less than 30 $mu$Bq/kg. The expected sensitivity to cosmic dark matter by using 250 kg of the high purity and large volume NaI(Tl) scintillator (PICO-LON; Pure Inorganic Crystal Observatory for LOw-background Neutr(al)ino) is 7$times$10$^{-45}$ cm$^{2}$ for 50 GeV$/c^{2}$ WIMPs.
The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The prog
enies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 pm1.4$ $mu$Bq/kg and $13pm4$ $mu$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $mu$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible.
We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the direct counting of radioactive $^{40}$K, is found to
be $2.2pm1.5$ ppb, lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1-6 keV energy region-of-interest (ROI) is $1.20pm0.05$ counts/day/kg/keV, which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by $^{210}$Pb and that about half of this contamination is located in the PTFE reflector. We discuss ongoing developments of the crystal manufacture aimed at the further reduction of the background, including data from purification by zone refining. A projected background rate lower than $sim$0.2 counts/day/kg/keV in the ROI is within reach. These results represent a benchmark for the development of next-generation NaI(Tl) detector arrays for the direct detection of dark matter particles.
Scintillating NaI(Tl) crystals are widely used in a large variety of experimental applications. However, for the use as Dark Matter (DM) detectors, such crystals demand a high level of radio-purity, not achievable by means of standard industrial tech
niques. One of the main difficulties comes from the presence of potassium that always accompanies sodium in alkali halides. On the other hand, the arguable DM detection by DAMA experiment using NaI(Tl) scintillating crystals requires a reliable verification able to either confirm the existence of DM or rule out the DAMA claim. Ultra-low radioactivity NaI(Tl) crystals, particularly with very low potassium content, are therefore indispensable to overcome the current stalemate in Dark Matter searches. Nonetheless, apart from DAMA-LIBRA experiments, to date, no other experiment has succeeded in building a detector from NaI(Tl) crystals with potassium content of ppb level. This work describes recent results in the preparation of ultra-radio-pure NaI(Tl) crystals using a modified Bridgman method. A double-walled platinum crucible technique has been designed and reliability tests show that 5 ppb of potassium in the NaI(Tl) crystals of 2 and 3 inches in diameter can be achieved starting from NaI powder with potassium content of the order of 10 ppb. The potassium excess is segregated in the tail-side of the as grown ingot where measured potassium concentration is above 20 ppb. The purifying effect of Bridgman growth for larger NaI(Tl) crystals is currently being tested. The work also reports on scintillation parameters of our NaI(Tl) crystals measured in a dedicated setup conceived for naked, hygroscopic crystals. The reproducible and reliable production of ultra-low radioactivity NaI(Tl) crystals reported in this work will hopefully spur the construction of new DM search experiments and, anyway, clarify the controversial DAMA-LIBRA results.
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