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Development of highly radiopure NaI(Tl) scintillator for PICOLON dark matter search project

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 نشر من قبل Ken-Ichi Fushimi
 تاريخ النشر 2021
  مجال البحث فيزياء
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The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 pm1.4$ $mu$Bq/kg and $13pm4$ $mu$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $mu$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible.

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A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl) crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $mu$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector module will be reported in this article.
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