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تسجيل مستخدم جديدFluctuation-Driven Selection at Criticality in a Frustrated Magnetic System: the Case of Multiple-k Partial Order on the Pyrochlore Lattice
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We study the problem of partially ordered phases with periodically arranged disordered (paramagnetic) sites on the pyrochlore lattice, a network of corner-sharing tetrahedra. The periodicity of these phases is characterized by one or more wave vectors k=(1/2 1/2 1/2). Starting from a general microscopic Hamiltonian including anisotropic nearest-neighbor exchange, long-range dipolar interactions and second- and third-nearest neighbor exchange, we identify using standard mean-field theory (s-MFT) an extended range of interaction parameters that support partially ordered phases. We demonstrate that thermal fluctuations ignored in s-MFT are responsible for the selection of one particular partially ordered phase, e.g. the 4-k phase over the 1-k phase. We suggest that the transition into the 4-k phase is continuous with its critical properties controlled by the cubic fixed point of a Ginzburg-Landau theory with a 4-component vector order-parameter. By combining an extension of the Thouless-Anderson-Palmer method originally used to study fluctuations in spin glasses with parallel-tempering Monte-Carlo simulations, we establish the phase diagram for different types of partially ordered phases. Our results elucidate the long-standing puzzle concerning the origin of the 4-k partially ordered phase observed in the Gd2Ti2O7 dipolar pyrochlore antiferromagnet below its paramagnetic phase transition temperature.
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Partially-ordered magnets are distinct from both spin liquids and conventional ordered magnets because order and disorder coexist in the same magnetic phase. Here, we determine the nature of partial order in the canonical frustrated pyrochlore antife
rromagnet Gd$_2$Ti$_{2}$O$_{7}$. Using single-crystal neutron-diffraction measurements in applied magnetic field, magnetic symmetry analysis, inelastic neutron-scattering measurements, and spin-wave modeling, we show that its low-temperature magnetic structure involves two propagation vectors (2-$mathbf{k}$ structure) with suppressed ordered magnetic moments and enhanced spin-wave fluctuations. Our experimental results support theoretical predictions of thermal fluctuation-driven order in Gd$_{2}$Ti$_{2}$O$_{7}$.
The frustrated pyrochlore antiferromagnet Gd$_{2}$Ti$_{2}$O$_{7}$ has an unusual partially-ordered magnetic structure at the lowest measurable temperatures. This structure is currently believed to involve four magnetic propagation vectors $mathbf{k}i
n langle frac{1}{2} frac{1}{2} frac{1}{2} rangle^*$ in a cubic 4-$mathbf{k}$ structure, based on analysis of magnetic diffuse-scattering data [J. Phys.: Condens. Matter 16, L321 (2004)]. Here, we present three pieces of evidence against the 4-$mathbf{k}$ structure. First, we report single-crystal neutron-diffraction measurements as a function of applied magnetic field, which are consistent with the selective field-induced population of non-cubic magnetic domains. Second, we present evidence from high-resolution powder neutron-diffraction measurements that rhombohedral strains exist within magnetic domains, which may be generated by magneto-elastic coupling only for the alternative 1-$mathbf{k}$ structure. Finally, we show that the argument previously used to rule out the 1-$mathbf{k}$ structure is flawed, and demonstrate that magnetic diffuse-scattering data can actually be fitted quantitatively by a 1-$mathbf{k}$ structure in which spin fluctuations on ordered and disordered magnetic sites are strongly coupled. Our results provide an experimental foundation on which to base theoretical descriptions of partially-ordered states.
Experimental evidence from measurements of the a.c. and d.c. susceptibility, and heat capacity data show that the pyrochlore structure oxide, Gd_2Ti_2O_7, exhibits short range order that starts developing at 30K, as well as long range magnetic order
at $Tsim 1$K. The Curie-Weiss temperature, $theta_{CW}$ = -9.6K, is largely due to exchange interactions. Deviations from the Curie-Weiss law occur below $sim$10K while magnetic heat capacity contributions are found at temperatures above 20K. A sharp maximum in the heat capacity at $T_c=0.97$K signals a transition to a long range ordered state, with the magnetic specific accounting for only $sim$ 50% of the magnetic entropy. The heat capacity above the phase transition can be modeled by assuming that a distribution of random fields acts on the $^8S_{7/2}$ ground state for Gd$^{3+}$. There is no frequency dependence to the a.c. susceptibility in either the short range or long range ordered regimes, hence suggesting the absence of any spin-glassy behavior. Mean field theoretical calculations show that no long range ordered ground state exists for the conditions of nearest-neighbor antiferromagnetic exchange and long range dipolar couplings. At the mean-field level, long range order at various commensurate or incommensurate wave vectors is found only upon inclusion of exchange interactions beyond nearest-neighbor exchange and dipolar coupling. The properties of Gd$_2Ti_2O_7 are compared with other geometrically frustrated antiferromagnets such as the Gd_3Ga_5O_{12} gadolinium gallium garnet, RE_2Ti_2O_7 pyrochlores where RE = Tb, Ho and Tm, and Heisenberg-type pyrochlore such as Y_2Mo_2O_7, Tb_2Mo_2O_7, and spinels such as ZnFe_2O_4
Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule governing th
e local ground state of a frustrated magnet. For example, the 2-in-2-out ice rule for dipole moments on a tetrahedron can lead to a quantum spin ice in rare-earth pyrochlores - a state described by a lattice gauge theory of quantum electrodynamics$^{2-4}$. However, f-electron ions often carry multipole degrees of freedom of higher rank than dipoles, leading to intriguing behaviours and hidden orders$^{5-6}$. Here we show that the correlated ground state of a Ce$^{3+}$-based pyrochlore, Ce$_2$Sn$_2$O$_7$, is a quantum liquid of magnetic octupoles. Our neutron scattering results are consistent with the formation of a fluid-like state of matter, but the intensity distribution is weighted to larger scattering vectors, which indicates that the correlated degrees of freedom have a more complex magnetization density than that typical of magnetic dipoles in a spin liquid. The temperature evolution of the bulk properties in the correlated regime below 1 Kelvin is well reproduced using a model of dipole-octupole doublets on a pyrochlore lattice$^{7-8}$. The nature and strength of the octupole-octupole couplings, together with the existence of a continuum of excitations attributed to spinons, provides further evidence for a quantum ice of octupoles governed by a 2-plus-2-minus rule. Our work identifies Ce$_2$Sn$_2$O$_7$ as a unique example of a material where frustrated multipoles form a hidden topological order, thus generalizing observations on quantum spin liquids to multipolar phases that can support novel types of emergent fields and excitations.
It was proposed in [(https://doi.org/10.1103/PhysRevLett.114.145301){Chen et al., Phys. Rev. Lett. $mathbf{114}$, 145301 (2015)}] that spin-2 chains display an extended critical phase with enhanced SU$(3)$ symmetry. This hypothesis is highly unexpect
ed for a spin-2 system and, as we argue, would imply an unconventional mechanism for symmetry emergence. Yet, the absence of convenient critical points for renormalization group perturbative expansions, allied with the usual difficulty in the convergence of numerical methods in critical or small-gapped phases, renders the verification of this hypothetical SU$(3)$-symmetric phase a non-trivial matter. By tracing parallels with the well-understood phase diagram of spin-1 chains and searching for signatures robust against finite-size effects, we draw criticism on the existence of this phase. We perform non-Abelian density matrix renormalization group studies of multipolar static correlation function, energy spectrum scaling, single-mode approximation, and entanglement spectrum to shed light on the problem. We determine that the hypothetical SU$(3)$ spin-2 phase is, in fact, dominated by ferro-octupolar correlations and also observe a lack of Luttinger-liquid-like behavior in correlation functions that suggests that is perhaps not critical. We further construct an infinite family of spin-$S$ systems with similar ferro-octupolar-dominated quasi-SU$(3)$-like phenomenology; curiously, we note that the spin-3 version of the problem is located in a subspace of exact G$_2$ symmetry, making this a point of interest for search of Fibonacci topological properties in magnetic systems.
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