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Measurements and calculations of the absolute carrier-envelope phase (CEP) effects in the photodissociation of the simplest molecule, H2+, with a 4.5-fs Ti:Sapphire laser pulse at intensities up to (4 +- 2)x10^14 Watt/cm^2 are presented. Localization of the electron with respect to the two nuclei (during the dissociation process) is controlled via the CEP of the ultra-short laser pulses. In contrast to previous CEP-dependent experiments with neutral molecules, the dissociation of the molecular ions is not preceded by a photoionization process, which strongly influences the CEP dependence. Kinematically complete data is obtained by time- and position-resolved coincidence detection. The phase dependence is determined by a single-shot phase measurement correlated to the detection of the dissoziation fragments. The experimental results show quantitative agreement with ab inito 3D-TDSE calculations that include nuclear vibration and rotation.
We present models for a heteronuclear diatomic molecular ion in a linear Paul trap in a rigid-rotor approximation, one purely classical, the other where the center-of-mass motion is treated classically while rotational motion is quantized. We study t
It is shown that the molecular ion ${rm H}^{++}_3$ does not exist in a form of the equilateral triangle. To this end, a compact variational method is presented which is based on a linear superposition of six specially tailored trial functions contain
We discuss and measure the phase shift imposed onto a radially polarized light beam when focusing it onto an $^{174}text{Yb}^{+}$ ion. In the derivation of the expected phase shifts we include the properties of the involved atomic levels. Furthermore
Trapped ions are a well-studied and promising system for the realization of a scalable quantum computer. Faster quantum gates would greatly improve the applicability of such a system and allow for greater flexibility in the number of calculation step
The application of a matrix-based reconstruction protocol for obtaining Molecular Frame (MF) photoelectron angular distributions (MFPADs) from laboratory frame (LF) measurements (LFPADs) is explored. Similarly to other recent works on the topic of MF