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We report nuclear magnetic resonance measurements of the spin-1/2 anisotropic triangular lattice antiferromagnet Cs$_2$CuCl$_4$ as a function of temperature and applied magnetic field. The observed temperature and magnetic field dependence of the NMR relaxation rate suggests that low energy excitations in the short-range ordered region stabilized over a wide range of intermediate fields and temperatures of the phase diagram are gapless or nearly gapless fermionic excitations. An upper bound on the size of the gap of 0.037 meV $approx J/10$ is established. The magnetization and NMR relaxation rate can be qualitatively described either by a quasi-1D picture of weakly coupled chains, or by mean-field theories of specific 2D spin liquids; however, quantitative differences exist between data and theory in both cases. This comparison indicates that 2D interactions are quantitatively important in describing the low-energy physics.
We report $^{133}$Cs nuclear magnetic resonance (NMR) measurements on the 2D frustrated Heisenberg antiferromagnet Cs$_2$CuCl$_4$ down to 2 K and up to 15 T. We show that $^{133}$Cs NMR is a good probe of the magnetic degrees of freedom in this mater
Quantum triangular-lattice antiferromagnets are important prototype systems to investigate phenomena of the geometrical frustration in condensed matter. Apart from highly unusual magnetic properties, they possess a rich phase diagram (ranging from an
We investigate the electronic and magnetic properties of the frustrated triangular-lattice antiferromagnets Cs$_2$CuCl$_4$ and Cs$_2$CuBr$_4$ in the framework of density functional theory. Analysis of the exchange couplings J and J using the availabl
We report on electron spin resonance (ESR) studies of the spin relaxation in Cs$_2$CuCl$_4$. The main source of the ESR linewidth at temperatures $T leq 150$ K is attributed to the uniform Dzyaloshinskii-Moriya interaction. The vector components of t
The spin excitations in the spin-liquid phase of the anisotropic triangular lattice quantum antiferromagnet Cs$_2$CuCl$_4$ have been shown to propagate dominantly along the crystallographic $b$ axis. To test this dimensional reduction scenario, we ha