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We report the observation of double-quantum coherence signals in a gas of potassium atoms at twice the frequency of the one-quantum coherences. Since a single atom does not have a state at the corresponding energy, this observation must be attributed to a collective resonance involving multiple atoms. These resonances are induced by weak inter-atomic dipole-dipole interactions, which means that the atoms cannot be treated in isolation, even at a low density of $10^{12}$ cm$^{-3}$.
Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The methods resolution makes multidimensional coherent spectroscopy relevant for atomic system
We experimentally and theoretically study two different tripod configurations using metastable helium ($^4$He*), with the probe field polarization perpendicular and parallel to the quantization axis, defined by an applied weak magnetic field. In the
We present an experimental and theoretical energy- and angle-resolved study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral N$_2$ molecules. Using 9.3 eV photons produced via high harmonic gen
Traditionally, measuring the center-of-mass (c.m.) velocity of an atomic ensemble relies on measuring the Doppler shift of the absorption spectrum of single atoms in the ensemble. Mapping out the velocity distribution of the ensemble is indispensable
The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes and chemical reactions. It is thus a long-standing scientific dream to measure the dynamics of two bound correlated electrons in the quantum re