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We present the results of a muon-spin relaxation study of the high-Tc analogue material Cs2AgF4. We find unambiguous evidence for magnetic order, intrinsic to the material, below T_C=13.95(3) K. The ratio of inter- to intraplane coupling is estimated to be |J/J|=1.9 x 10^-2, while fits of the temperature dependence of the order parameter reveal a critical exponent beta=0.292(3), implying an intermediate character between pure two- and three- dimensional magnetism in the critical regime. Above T_C we observe a signal characteristic of dipolar interactions due to linear F-mu-F bonds, allowing the muon stopping sites in this compound to be characterized.
We present the results of muon-spin relaxation (muSR) measurements on the hexagonal manganite HoMnO3. Features in the temperature-dependent relaxation rate, lambda, correlate with the magnetic transitions at 76 K, 38 K and 34 K. The highest temperatu
We present longitudinal field muon spin relaxation ($mu$SR) measurements in the unilluminated state of the photo-sensitive molecular magnetic Co-Fe Prussian blue analogues M$_{1-2x}$Co$_{1+x}$[Fe(CN)$_6$]$cdot z$ H$_2$O, where M=K and Rb with $x=0.4$
We demonstrate that quantum-critical spin dynamics can be probed in high magnetic fields using muon-spin relaxation ($mu^{+}$SR). Our model system is the strong-leg spin ladder bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). In the gapless Tom
Although the precise mechanism of high-Tc superconductivity in the layered cuprates remains unknown, it is generally thought that strong 2D Heisenberg antiferromagnetism combined with disruptive hole doping is an essential aspect of the phenomenon. I
We review examples of muon-spin relaxation measurements on molecule-based magnetic coordination polymers, classified by their magnetic dimensionality. These include the one-dimensional s=1/2 spin chain Cu(pyz)(NO3)2 and the two-dimensional s=1/2 laye