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تسجيل مستخدم جديدSpin-Flop Transition and Anisotropic Magnetoresistance in Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4}: Unexpectedly Strong Spin-Charge Coupling in Electron-Doped Cuprates
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We use transport and neutron-scattering measurements to show that a magnetic-field-induced transition from noncollinear to collinear spin arrangement in adjacent CuO_{2} planes of lightly electron-doped Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4} (x=0.01) crystals affects significantly both the in-plane and out-of-plane resistivity. In the high-field collinear state, the magnetoresistance (MR) does not saturate, but exhibits an intriguing four-fold-symmetric angular dependence, oscillating from being positive at B//[100] to being negative at B//[110]. The observed MR of more than 30% at low temperatures induced by a modest modification of the spin structure indicates an unexpectedly strong spin-charge coupling in electron-doped cuprates.
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The pairing state symmetry of the electron-doped cuprate superconductors is thought to be s-wave in nature, in contrast with their hole-doped counterparts which exhibit a d-wave symmetry. We re-examine this issue based on recent improvements in our e
lectron-doped materials and our measurement techniques. We report microwave cavity perturbation measurements of the temperature dependence of the penetration depth of Pr_(2-x)Ce_(x)CuO_(4-y) and Nd_(2-x)Ce_(x)CuO_(4-y) crystals. Our data strongly suggest that the pairing symmetry in these materials is not s-wave.
It was recently demonstrated that the anisotropic phonon heat transport behavior is a good probe of the stripe formation in La_{2-x}Sr_xCuO_4 (LSCO) [X. F. Sun {it et al.}, Phys. Rev. B {bf 67}, 104503 (2003)]. Using this probe, we examined an electr
on-doped cuprate Pr_{1.3-x}La_{0.7}Ce_xCuO_4 (PLCCO) and found that essentially the same features as those in LSCO are observed. Moreover, the in-plane resistivity rho_{ab} of lightly-doped PLCCO shows metallic behavior (drho_{ab}/dT > 0) in the Neel ordered state with a mobility comparable to that in LSCO. It is discussed that these peculiar properties in common with LSCO signify the existence of stripes in electron-doped cuprates.
We present a detailed temperature-dependent Raman light scattering study of optical phonons in molecular-beam-epitaxy-grown films of the electron-doped superconductor La_{2-x}Ce_{x}CuO_{4} close to optimal doping (x ~ 0.08, T_c = 29 K and x ~ 0.1, T_
c = 27 K). The main focus of this work is a detailed characterization and microstructural analysis of the films. Based on micro-Raman spectroscopy in combination with x-ray diffraction, energy-dispersive x-ray analysis, and scanning electron microscopy, some of the observed phonon modes can be attributed to micron-sized inclusions of Cu_{2}O. In the slightly underdoped film (x ~ 0.08), both the Cu_{2}O modes and others that can be assigned to the La_{2-x}Ce_{x}CuO_{4} matrix show pronounced softening and narrowing upon cooling below T ~ T_c. Based on control measurements on commercial Cu_{2}O powders and on a comparison to prior Raman scattering studies of other high-temperature superconductors, we speculate that proximity effects at La_{2-x}Ce_{x}CuO_{4}/Cu_{2}O interfaces may be responsible for these anomalies. Experiments on the slightly overdoped La_{2-x}Ce_{x}CuO_{4} film (x ~ 0.1) did not reveal comparable phonon anomalies.
Superstructure reflections due to the ordering of holes into stripes in La_(1.45)Nd_(0.4)Sr_(0.15)CuO_4 have been studied with high energy x-ray diffraction. These reflections have been observed clearly for the first time in a sample which is superco
nducting at low temperatures (T_c = 10 K). The stripe peaks vanish above 62(5) K whereas the magnetic signal of the stripe ordering which has been seen with neutrons before is already suppressed at 45 K. Our results confirm that the ordering of spins and holes is driven by the charges as it is found in the case of La_(1.6-x)Nd_(0.4)Sr_(x)CuO_(4) at the doping level of x = 0.12.
For electron-doped cuprates, the strong suppression of antiferromagnetic spin correlation by efficient reduction annealing by the protect-annealing method leads to superconductivity not only with lower Ce concentrations but also with higher transitio
n temperatures. To reveal the nature of this superconducting state, we have performed angle-resolved photoemission spectroscopy measurements of protect-annealed electron-doped superconductors Pr$_{1.3-x}$La$_{0.7}$Ce$_{x}$CuO$_{4}$ and directly investigated the superconducting gap. The gap was found to be consistent with $d$-wave symmetry, suggesting that strong electron correlation persists and hence antiferromagnetic spin fluctuations remain a candidate that mediates Copper pairing in the protect-annealed electron-doped cuprates.
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