ترغب بنشر مسار تعليمي؟ اضغط هنا

Glassy Spin Dynamics in Non-Fermi-Liquid UCu_{5-x}Pd_x, x = 1.0 and 1.5

70   0   0.0 ( 0 )
 نشر من قبل Douglas E. MacLaughlin
 تاريخ النشر 2000
  مجال البحث فيزياء
والبحث باللغة English
 تأليف D. E. MacLaughlin




اسأل ChatGPT حول البحث

Local f-electron spin dynamics in the non-Fermi-liquid heavy-fermion alloys UCu_{5-x}Pd_x, x = 1.0 and 1.5, have been studied using muon spin-lattice relaxation. The sample-averaged asymmetry function Gbar(t) indicates strongly inhomogeneous spin fluctuations, and exhibits the scaling Gbar(t,H) = Gbar(t/H^gamma) expected from glassy dynamics. At 0.05 K gamma(x=1.0) = 0.35 pm 0.1, but gamma(x=1.5) = 0.7 pm 0.1. This is in contrast to inelastic neutron scattering results, which yield gamma = 0.33 for both concentrations. There is no sign of static magnetism gtrsim 10^{-3} mu_B/U ion in either material above 0.05 K. Our results strongy suggest that both alloys are quantum spin glasses.

قيم البحث

اقرأ أيضاً

Low-temperature muon spin-lattice relaxation measurements in the non-Fermi-liquid heavy-fermion alloys UCu_{5-x}Pd_x, x = 1.0 and 1.5, indicate inhomogeneously distributed f-electron spin fluctuation rates, and exhibit a time-field scaling of the muo n relaxation function indicative of long-lived spin correlations. In UCu_4Pd the scaling exponent gamma is small and temperature independent. In UCu_{3.5}Pd_{1.5} gamma varies with temperature, increasing with decreasing temperature similar to spin-glass AgMn. This suggests that the spin-glass state found for x gtrsim 2 in UCu_{5-x}Pd_x modifies the low-frequency spin dynamics in UCu_{3.5}Pd_{1.5}.
Longitudinal-field muon spin relaxation (LF-muSR) experiments have been performed in unannealed and annealed samples of the heavy-fermion compound UCu_4Pd to study the effect of disorder on non-Fermi liquid behavior in this material. The muon spin re laxation functions G(t,H) obey the time-field scaling relation G(t,H) = G(t/H^gamma) previously observed in this compound. The observed scaling exponent gamma = 0.3 pm 0.1, independent of annealing. Fits of the stretched-exponential relaxation function G(t) = exp[-(Lambda t)^K] to the data yielded stretching exponentials K < 1 for all samples. Annealed samples exhibited a reduction of the relaxation rate at low temperatures, indicating that annealing shifts fluctuation noise power to higher frequencies. There was no tendency of the inhomogeneous spread in rates to decrease with annealing, which modifies but does not eliminate the glassy spin dynamics reported previously in this compound. The correlation with residual resistivity previously observed for a number of NFL heavy-electron materials is also found in the present work.
The non-Fermi liquid system (NFL) YbCu_(5-x)Al_(x) (x = 1.3 - 1.75) has been investigated in hetero- as well as homo-contact arrangement in magnetic fields up to 22.5 T. The observed dV/dI(V) characteristics reveal asymmetry in hetero-contact arrange ment and do not agree with the model of thermal contact heating, at least close to zero-bias voltage. In the case of a hetero-contact arrangement we have observed a maximum at only one voltage polarity at about 1.3 mV (for x = 1.5), which asymmetry is suppressed in an applied magnetic field. This behavior is connected with NFL properties of studied compounds.
Muon spin rotation and relaxation ($mu$SR) experiments have yielded evidence that structural disorder is an important factor in many f-electron-based non-Fermi-liquid (NFL) systems. Disorder-driven mechanisms for NFL behaviour are suggested by the ob served broad and strongly temperature-dependent $mu$SR (and NMR) linewidths in several NFL compounds and alloys. Local disorder-driven theories (Kondo disorder, Griffiths-McCoy singularity) are, however, not capable of describing the time-field scaling seen in muon spin relaxation experiments, which suggest cooperative and critical spin fluctuations rather than a distribution of local fluctuation rates. A strong empirical correlation is established between electronic disorder and slow spin fluctuations in NFL materials
The evolution of the Fermi surface of CeRh$_{1-x}$Co$_x$In$_5$ was studied as a function of Co concentration $x$ via measurements of the de Haas-van Alphen effect. By measuring the angular dependence of quantum oscillation frequencies, we identify a Fermi surface sheet with $f$-electron character which undergoes an abrupt change in topology as $x$ is varied. Surprisingly, this reconstruction does not occur at the quantum critical concentration $x_c$, where antiferromagnetism is suppressed to T=0. Instead we establish that this sudden change occurs well below $x_c$, at the concentration x ~ 0.4 where long range magnetic order alters its character and superconductivity appears. Across all concentrations, the cyclotron effective mass of this sheet does not diverge, suggesting that critical behavior is not exhibited equally on all parts of the Fermi surface.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا