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تسجيل مستخدم جديدReal-space nanoimaging of THz polaritons in the topological insulator Bi2Se3
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Dirac plasmon polaritons in topological insulators (TIs),light coupled to massless Dirac electrons, have been attracting a large amount of attention, both from a fundamental perspective and for potential terahertz (THz) photonic applications. Although THz polaritons have been observed by far-field THz spectroscopy on TI microstructures, real-space imaging of propagating THz polaritons in unstructured TIs has been elusive so far. Here, we show the very first spectroscopic THz near-field images of thin Bi2Se3 layers (prototypical TIs) revealing polaritons with up to 12 times increased momenta as compared to photons of the same energy and decay times of about 0.24 ps, yet short propagation lengths. From the near-field images we determine the polariton dispersions in layers from 120 to 25 nm thickness and perform a systematic theoretical dispersion analysis, showing that the observed polaritons can be explained only by the simultaneous coupling of THz radiation to Dirac carriers at the TI surfaces, massive bulk carriers and optical phonons. Our work does not only provide critical insights into the nature of THz polaritons in TIs, but also establishes instrumentation of unprecedented sensitivity for imaging of THz polaritons.
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