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We have performed angle-resolved photoemission spectroscopy on epitaxial VTe2 films to elucidate the relationship between the fermiology and charge-density waves (CDW). We found that a two-dimensional triangular pocket in 1 monolayer (ML) VTe2 is converted to a strongly warped quasi-one-dimensional (1D) Fermi surface in the 6ML counterpart, likely associated with the 1T-to-1T structural phase transition. We also revealed a metallic Fermi edge on the entire Fermi surface in 6ML at low temperature distinct from anisotropic pseudogap in 1ML, signifying a contrast behavior of CDW that is also supported by first-principles band-structure caluculations. The present result points to the importance of simultaneously controlling the structural phase and fermiology to manipulate the CDW properties in ultrathin transition-metal dichalcogenides.
The concept of a CDW induced by Fermi-surface nesting originated from the Peierls idea of electronic instabilities in purely 1D metals and is now often applied to charge ordering in real low-dimensional materials. The idea is that if Fermi surface co
We investigate the three-dimensional electronic structure of the seminal charge-density-wave (CDW) material 2H-NbSe$_2$ by soft x-ray angle-resolved photoelectron spectroscopy and density-functional theory. Our results reveal the pronounced 3D charac
Charge, spin, as well as lattice instabilities are investigated in isolated or weakly coupled chains of correlated electrons at quarter-filling. Our analysis is based on extended Hubbard models including nearest neighbor repulsion and Peierls couplin
We have thoroughly characterized the surfaces of the organic charge-transfer salts TTF-TCNQ and (TMTSF)2PF6 which are generally acknowledged as prototypical examples of one-dimensional conductors. In particular x-ray induced photoemission spectroscop
Ta2NiSe7 is a quasi-one-dimensional (quasi-1D) transition-metal chalcogenide with Ta and Ni chain structure. An incommensurate charge-density wave (CDW) in this quasi-1D structure was well studied previously using tunnelling spectrum, X-ray and elect