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تسجيل مستخدم جديدDiscovery of an ultra-quantum spin liquid
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Quantum fluctuations are expected to lead to highly entangled spin-liquid states in some two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon relaxation rates in Cu-based two-dimensional triangular-lattice spin liquids, one of which is the least disordered of this kind synthesized hitherto. Its measured properties can all be simply characterized by scale-invariant time-dependent fluctuations with a single parameter. The specific heat divided by temperature and muon relaxation rates are both temperature-independent at low temperatures, followed by a logarithmic decrease with increasing temperature. Even more remarkably, $sim$57% of the magnetic entropy is missing down to temperatures of textit{O}(10$^{-3}$) the exchange energy, independent of magnetic field up to $gmu_BH > k_BT$@. These properties are intrinsic. They are evidence that quantum fluctuations lead either to a gigantic specific heat peak from topological singlet excitations below such temperatures, or to an extensively degenerate topological singlet ground state. This is an ultra-quantum state of matter.
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A quantum spin liquid (QSL) is an exotic state of matter in which electrons spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a central ai
m of experimental physics, because they host collective excitations that transcend our knowledge of quantum matter; however, examples in real materials are scarce. Here, we report neutron-scattering measurements on YbMgGaO4, a QSL candidate in which Yb3+ ions with effective spin-1/2 occupy a triangular lattice. Our measurements reveal a continuum of magnetic excitations - the essential experimental hallmark of a QSL - at very low temperature (0.06 K). The origin of this peculiar excitation spectrum is a crucial question, because isotropic nearest-neighbor interactions do not yield a QSL ground state on the triangular lattice. Using measurements of the magnetic excitations close to the field-polarized state, we identify antiferromagnetic next-nearest-neighbor interactions in the presence of planar anisotropy as key ingredients for QSL formation in YbMgGaO4.
Two-dimensional triangular-lattice materials with spin-1/2 are perfect platforms for investigating quantum frustrated physics with spin fluctuations. Here we report the structure, magnetization, heat capacity and inelastic neutron scattering (INS) re
sults on cesium ytterbium diselenide, CsYbSe$_2$. There is no long-range magnetic order down to 0.4 K at zero field. The temperature dependent magnetization, $M(T)$, reveals an easy-plane magnetic anisotropy. A maximum is found in $M(T)$ around emph{T}$sim$1.5 K when magnetic field $H$ is applied in the $ab$ plane, indicating the short-range interaction. The low-temperature isothermal magnetization $M(H)$ shows a one-third plateau of the estimated saturation moment, that is characteristic of a two-dimensional frustrated triangular lattice. Heat capacity shows field-induced long-range magnetic order for both $H||c$ and $H||ab$ directions. The broad peak in heat capacity and highly damped INS magnetic excitation at $T$=2 K suggests strong spin fluctuations. The dispersive in-plane INS, centered at the (1/3 1/3 0) point, and the absence of dispersion along $c$ direction suggests 120$^{circ}$ non-collinear 2D-like spin correlations. All these results indicate that the two-dimensional frustrated material CsYbSe$_2$ can be in proximity to the triangular-lattice quantum spin liquid. We propose an experimental low-temperature $H$-$T$ phase diagram for CsYbSe$_2$.
Arguably the most favorable situation for spins to enter the long-sought quantum spin liquid (QSL) state is when they sit on a kagome lattice. No consensus has been reached in theory regarding the true ground state of this promising platform. The exp
erimental efforts, relying mostly on one archetypal material ZnCu$_3$(OH)$_6$Cl$_2$, have also led to diverse possibilities. Apart from subtle interactions in the Hamiltonian, there is the additional degree of complexity associated with disorder in the real material ZnCu$_3$(OH)$_6$Cl$_2$ that haunts most experimental probes. Here we resort to heat transport measurement, a cleaner probe in which instead of contributing directly, the disorder only impacts the signal from the kagome spins. For ZnCu$_3$(OH)$_6$Cl$_2$ and a related QSL candidate Cu$_3$Zn(OH)$_6$FBr, we observed no contribution by any spin excitation nor any field-induced change to the thermal conductivity. These results impose different constraints on various scenarios about the ground state of these two kagome compounds: while a gapped QSL, or certain quantum paramagnetic state other than a QSL, is compatible with our results, a gapless QSL must be dramatically modified by the disorder so that gapless spin excitations are localized.
Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are hypothetically associat
ed with quasiparticle fractionalization and topological order. Here we report highly unusual heat conduction generated by the spin degrees of freedom in a QSL state of the pyrochlore magnet Pr$_2$Zr$_2$O$_7$, which hosts spin-ice correlations with strong quantum fluctuations. The thermal conductivity in high temperature regime exhibits a two-gap behavior, which is consistent with the gapped excitations of magnetic ($M$-) and electric monopoles ($E$-particles). At very low temperatures below 200,mK, the thermal conductivity unexpectedly shows a dramatic enhancement, which well exceeds purely phononic conductivity, demonstrating the presence of highly mobile spin excitations. This new type of excitations can be attributed to emergent photons ($ u$-particle), coherent gapless spin excitations in a spin-ice manifold.
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