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Recently monolayer jacutingaite (Pt2HgSe3), a naturally occurring exfoliable mineral, discovered in Brazil in 2008, has been theoretically predicted as a candidate quantum spin Hall system with a 0.5 eV band gap, while the bulk form is one of only a few known dual-topological insulators which may host different surface states protected by symmetries. In this work, we systematically investigate both structure and electronic evolution of bulk Pt2HgSe3 under high pressure up to 96 GPa. The nontrivial topology persists up to the structural phase transition observed in the high-pressure regime. Interestingly, we found that this phase transition is accompanied by the appearance of superconductivity at around 55 GPa and the critical transition temperature Tc increases with applied pressure. Our results demonstrate that Pt2HgSe3 with nontrivial topology of electronic states displays new ground states upon compression and raises potentials in application to the next-generation spintronic devices.
Topological nodal-line semimetals (TNLSMs) are materials whose conduction and valence bands cross each other, meeting a topologically-protected closed loop rather than discrete points in the Brillouin zone (BZ). The anticipated properties for TNLSMs
Topological superconductivity with Majorana bound states, which are critical to implement nonabelian quantum computation, may be realized in three-dimensional semimetals with nontrivial topological feature, when superconducting transition occurs in t
Chemical doping of topological materials may provide a possible route for realizing topological superconductivity. However, all such cases known so far are based on chalcogenides. Here we report the discovery of superconductivity induced by Re doping
Bi2Te3 compound has been theoretically predicted (1) to be a topological insulator, and its topologically non-trivial surface state with a single Dirac cone has been observed in photoemission experiments (2). Here we report that superconductivity (Tc
The recently discovered Dirac and Weyl semimetals are new members of topological materials. Starting from them, topological superconductivity may be achieved, e.g. by carrier doping or applying pressure. Here we report high-pressure resistance and X-