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Here we report on the formation of two and three magnon bound states in the quasi-one-dimensional antiferromagnet $alpha$-NaMnO$_2$, where the single-ion, uniaxial anisotropy inherent to the Mn$^{3+}$ ions in this material provides a binding mechanism capable of stabilizing higher order magnon bound states. While such states have long remained elusive in studies of antiferromagnetic chains, neutron scattering data presented here demonstrate that higher order $n>2$ composite magnons exist, and, specifically, that a weak three-magnon bound state is detected below the antiferromagnetic ordering transition of NaMnO$_2$. We corroborate our findings with exact numerical simulations of a one-dimensional Heisenberg chain with easy-axis anisotropy using matrix-product state techniques, finding a good quantitative agreement with the experiment. These results establish $alpha$-NaMnO$_2$ as a unique platform for exploring the dynamics of composite magnon states inherent to a classical antiferromagnetic spin chain with Ising-like single ion anisotropy.
Spin-waves e.g. magnons are the conventional elementary excitations of ordered magnets. However, other possibilities exist. For instance, magnon bound-states can arise due to attractive magnon-magnon interactions and drastically impact the static and
We report $^{51}$V nuclear magnetic resonance (NMR) and inelastic neutron scattering (INS) measurements on a quasi-1D antiferromagnet BaCo$_2$V$_2$O$_8$ under transverse field along the [010] direction. The scaling behavior of the spin-lattice relaxa
Combining inelastic neutron scattering and numerical simulations, we study the quasi-one dimensional Ising anisotropic quantum antiferromagnet bacovo in a longitudinal magnetic field. This material shows a quantum phase transition from a Neel ordered
Magnetization measurements on single-crystal cubic SrCuTe$_2$O$_6$ with an applied magnetic field of along three inequivalent high symmetry directions $[100]$, $[110]$, and $[111]$ reveal weak magnetic anisotropy. The fits of the magnetic susceptibil
Quasi-one-dimensional iron-based ladders and chains, with the 3$d$ iron electronic density $n = 6$, are attracting considerable attention. Recently, a new iron chain system Ba$_2$FeS$_3$, also with $n = 6$, was prepared under high-pressure and high-t