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تسجيل مستخدم جديدAtomic manipulation of the gap in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$
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Single atom manipulation within doped correlated electron systems would be highly beneficial to disentangle the influence of dopants, structural defects and crystallographic characteristics on their local electronic states. Unfortunately, their high diffusion barrier prevents conventional manipulation techniques. Here, we demonstrate the possibility to reversibly manipulate select sites in the optimally doped high temperature superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ using the local electric field of the tip. We show that upon shifting individual Bi atoms at the surface, the spectral gap associated with superconductivity is seen to reversibly change by as much as 15 meV (~5% of the total gap size). Our toy model that captures all observed characteristics suggests the field induces lateral movement of point-like objects that create a local pairing potential in the CuO2 plane.
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The quantum condensate of Cooper-pairs forming a superconductor was originally conceived to be translationally invariant. In theory, however, pairs can exist with finite momentum $Q$ and thereby generate states with spatially modulating Cooper-pair d
ensity. While never observed directly in any superconductor, such a state has been created in ultra-cold $^{6}$Li gas. It is now widely hypothesized that the cuprate pseudogap phase contains such a pair density wave (PDW) state. Here we use nanometer resolution scanned Josephson tunneling microscopy (SJTM) to image Cooper-pair tunneling from a $d$-wave superconducting STM tip to the condensate of Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$. Condensate visualization capabilities are demonstrated directly using the Cooper-pair density variations surrounding Zn impurity atoms and at the Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ crystal-supermodulation. Then, by using Fourier analysis of SJTM images, we discover the direct signature of a Cooper-pair density modulation at wavevectors $Q_{p} approx (0.25,0)2pi / a_{0}$;$(0,0.25)2pi / a_{0}$ in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$. The amplitude of these modulations is ~5% of the homogenous condensate density and their form factor exhibits primarily $s$/$s$-symmetry. This phenomenology is expected within Ginzburg-Landau theory when a charge density wave with $d$-symmetry form factor and wave vector $Q_{c}=Q_{p}$ coexists with a homogeneous $d$-symmetry superconductor ; it is also encompassed by several contemporary microscopic theories for the pseudogap phase.
Varying the superconducting transition temperature over a large scale of a cuprate superconductor is a necessary step for identifying the unsettled mechanism of superconductivity. Chemical doping or element substitution has been proven to be effectiv
e but also brings about lattice disorder. Such disorder can completely destroy superconductivity even at a fixed doping level. Pressure has been thought to be the most clean method for tuning superconductivity. However, pressure-induced increase of disorder was recognized from recent experiments. By choosing a disordered Tl$_{2}$Ba$_{2}$CaCu$_{2}$O$_{8+delta}$ at the optimal doping, we perform single-crystal x-ray diffraction and magnetic susceptibility measurements at high pressures. The obtained structural data provides evidence for the robust feature for the disorder of this material in the pressure range studied. This feature ensures the pressure effects on superconductivity distinguishable from the disorder. The derived parabolic-like behavior of the transition temperature with pressure up to near 30 GPa, having a maximum around 7 GPa, offers a platform for testing any realistic theoretical models in a nearly constant disorder environment. Such a behavior can be understood when considering the carrier concentration and the pairing interaction strength as two pressure intrinsic variables.
High-quality Bi$_{2-x}$Pb$_{x}$Sr$_2$CaCu$_2$O$_{8+delta}$ (Bi2212) single crystals have been successfully grown by the traveling solvent floating zone technique with a wide range of Pb substitution ($x=0-0.8$). The samples are characterized by trans
mission electron microscope (TEM) and measured by high resolution laser-based angle-resolved photoemission spectroscopy (ARPES) with different photon energies. A systematic evolution of the electronic structure and superstructure with Pb substitution has been revealed for the first time. The superstructure shows a significant change with Pb substitution and the incommensurate modulation vector ($textbf{Q}$) decreases with increasing Pb substitution. In the meantime, the superstructure intensity from ARPES measurements also decreases dramatically with increasing Pb concentration. The superstructure in Bi2212 can be effectively suppressed by Pb substitution and it nearly disappears with a Pb substitution of $x=0.8$. We also find that the superstructure bands in ARPES measurements depend sensitively on the photon energy of lasers used; they can become even stronger than the main band when using a laser photon energy of 10.897 eV. These results provide important information on the origin of the incommensurate superstructure and its control and suppression in bismuth-based high temperature superconductors.
Scanning Hall probe and local Hall magnetometry measurements have been used to investigate flux distributions in large mesoscopic superconducting disks with sizes that lie near the crossover between the bulk and mesoscopic vortex regimes. Results obt
ained by directly mapping the magnetic induction profiles of the disks at different applied fields can be quite successfully fitted to analytic models which assume a continuous distribution of flux in the sample. At low fields, however, we do observe clear signatures of the underlying discrete vortex structure and can resolve the characteristic mesoscopic compression of vortex clusters in increasing magnetic fields. Even at higher fields, where single vortex resolution is lost, we are still able to track configurational changes in the vortex patterns, since competing vortex orders impose unmistakable signatures on local magnetisation curves as a function of the applied field. Our observations are in excellent agreement with molecular dynamics numerical simulations which lead us to a natural definition of the lengthscale for the crossover between discrete and continuum behaviours in our system.
Anomalously high and sharp peaks in the conductance of intrinsic Josephson junctions in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+delta}$ (Bi2212) mesas have been universally interpreted as superconducting energy gaps, but here we show they are a result of hea
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