ﻻ يوجد ملخص باللغة العربية
We present a joint experimental and theoretical study of spin coherence properties of 39K, 85Rb, 87Rb, and 133Cs atoms trapped in a solid parahydrogen matrix. We use optical pumping to prepare the spin states of the implanted atoms and circular dichroism to measure their spin states. Optical pumping signals show order-of-magnitude differences depending on both matrix growth conditions and atomic species. We measure the ensemble transverse relaxation times (T2*) of the spin states of the alkali-metal atoms. Different alkali species exhibit dramatically different T2* times, ranging from sub-microsecond coherence times for high mF states of 87Rb, to ~100 microseconds for 39K. These are the longest ensemble T2* times reported for an electron spin system at high densities (n > 10^16 cm^-3). To interpret these observations, we develop a theory of inhomogenous broadening of hyperfine transitions of ^2S atoms in weakly-interacting solid matrices. Our calculated ensemble transverse relaxation times agree well with experiment, and suggest ways to longer coherence times in future work.
Coherence time is an essential parameter for quantum sensing, quantum information, and quantum computation. In this work, we demonstrate electron spin coherence times as long as 0.1 s for an ensemble of rubidium atoms trapped in a solid parahydrogen
It is known from ensemble measurements that rubidium atoms trapped in solid parahydrogen have favorable properties for quantum sensing of magnetic fields. To use a single rubidium atom as a quantum sensor requires a technique capable of efficiently m
We present calculations of spin-relaxation rates of alkali-metal atoms due to the spin-axis interaction acting in binary collisions between the atoms. We show that for the high-temperature conditions of interest here, the spin relaxation rates calcul
We study the van der Waals interaction between Rydberg alkali-metal atoms with fine structure ($n^2L_j$; $Lleq 2$) and heteronuclear alkali-metal dimers in the ground rovibrational state ($X^1Sigma^+$; $v=0$, $J=0$). We compute the associated $C_6$ d
We present a versatile and compact electron beam driven source for alkali metal atoms, which can be implemented in cryostats. With a heat load of less than 10mW, the heat dissipation normalized to the atoms loaded into the magneto-optical Trap (MOT),