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The spin-driven component of electric polarization in a single crystal of multiferroic BiFeO$_{3}$ was experimentally investigated in pulsed high magnetic fields up to 41 T. Sequential measurements of electric polarization for various magnetic field directions provide clear evidence of electric polarization normal to the hexagonal $c$ axis (${bf P}_{rm t}$) in not only the cycloidal phase, but also the field-induced canted antiferromagnetic phase. The direction of ${bf P}_{rm t}$ is directly coupled with the ferromagnetic moment in the canted antiferromagnetic phase, and thus controlled by changing the direction of the applied magnetic field. This magnetoelectric coupling is reasonably reproduced by the metal-ligand hybridization model.
We report the results of direct measurement of remanent hysteresis loops on nanochains of BiFeO$_3$ at room temperature under zero and $sim$20 kOe magnetic field. We noticed a suppression of remanent polarization by nearly $sim$40% under the magnetic
We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman spectra ha
We investigate the temperature-dependent electronic structure of the van der Waals ferromagnet, CrGeTe$_3$. Using angle-resolved photoemission spectroscopy, we identify atomic- and orbital-specific band shifts upon cooling through ${T_mathrm{C}}$. Fr
Using THz spectroscopy, we show that the spin-wave spectrum of multiferroic BiFeO$_3$ in its high-field canted antiferromagnetic state is well described by a spin model that violates rhombohedral symmetry. We demonstrate that the monoclinic distortio
We have studied the magnetic field dependence of far-infrared active magnetic modes in a single ferroelectric domain BFO/ crystal at low temperature. The modes soften close to the critical field of 18.8,T along the [001] (pseudocubic) axis, where the